Journal
ORGANIC LETTERS
Volume 12, Issue 13, Pages 2978-2981Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol101002b
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Funding
- NIH [GM069559]
- Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division, US Department of Energy [DE-AC02-05CH11231]
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An efficient method is reported for the preparation of multicyclic pyridines and quinolines by a rhodium-catalyzed intramolecular C H bond functionalization process. The method shows good scope for branched and unbranched alkyl substituents on the pyridine ring and at the R position of the tethered alkene group. Starting materials capable of undergoing olefin isomerization to provide terminal 1,1-disubstituted alkenes also proved to be effective substrates.
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