Journal
ORGANIC LETTERS
Volume 10, Issue 20, Pages 4561-4564Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol8017775
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Funding
- National Institutes of Health [GM 46059, GM 1S10RR-13886-01]
- Merck
- Amgen
- Boehringer-Ingelheim
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An improved protocol for the Pd-catalyzed alpha-arylation of aldehydes with aryl halides has been developed. The new catalytic system allows for the coupling of an array of substrates including challenging electron-rich aryl bromides and less reactive aryl chlorides. The utility of this method has been demonstrated in a new total synthesis of (+/-)-sporochnol.
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