4.6 Article

Eigen oscillations of a chiral sphere and their influence on radiation of chiral molecules

Journal

OPTICS EXPRESS
Volume 22, Issue 15, Pages 18564-18578

Publisher

Optica Publishing Group
DOI: 10.1364/OE.22.018564

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Funding

  1. Russian Foundation [11-02-91065, 11-02-92002, 11-02-01272, 12-02-90014, 14-02-00290]
  2. Presidium of the Russian Academy of Sciences
  3. Russian Quantum Center
  4. Skolkovo Foundation

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Eigenmodes of a chiral sphere placed in a dielectric medium were investigated in details. Excitation of these eigenmodes by a plane wave and a chiral molecule radiation was studied both analytically and numerically. It was found that decay rates of right and left enantiomers are different in the presence of the chiral sphere. Strong dependence of radiation pattern of the chiral molecule placed in the vicinity of the chiral sphere on chirality strength was also demonstrated. An interesting correlation between chirality of sphere and spatial spirality (helicity, vorticity ...) of the electromagnetic fields in the presence of chiral sphere was observed for the first time. (C) 2014 Optical Society of America

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