Journal
SYNLETT
Volume 27, Issue 4, Pages 586-590Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0035-1560485
Keywords
chiral phosphoric acid; Friedel-Crafts reaction; pyrrole; sequential catalysis; tetrahydroindolizine; Zhan-1B
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Funding
- National Basic Research Program of China (973 Program) [2015CB856600]
- National Natural Science Foundation of China [21272253, 21332009, 21421091]
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A chiral phosphoric acid and a ruthenium complex were found to catalyze an olefin cross-metathesis-asymmetric intramolecular Friedel-Crafts alkylation of N-tethered olefin pyrroles and conjugated enones to provide a variety of chiral tetrahydroindolizine derivatives in moderate to good yields and enantioselectivity (up to 93% ee).
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