Journal
NANOSCALE
Volume 10, Issue 18, Pages 8772-8778Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8nr01336e
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Funding
- National Key R&D Program of China [2017YFA0207201]
- National Natural Science Foundation of China [21376190, 21676215, 21574065, 21604038, 51702155]
- Shaanxi Provincial Postdoctoral Science Special Foundation [2014-907]
- Shaanxi Provincial Science Foundation [2014SZS07-Z02, 2017SF-201]
- Scientific Research Program of Shaanxi Provincial Department of Education [15JS104]
- National Science Funds for Distinguished Young Scholars [21625401]
- Jiangsu Provincial Funds for Natural Science Foundation [BK20160975, BK20170975]
- Program for Outstanding Young Scholars from Organization Department of the CPC Central Committee
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Multicomponent metal-organic framework (MOF) derivatives have attracted strong interest in energy and environmental fields. However, most of the papers focus on single MOF derivatives; reports on multicomponent MOF derivatives and their catalytic studies are relatively few. Here, we report an easy-to-operate strategy to obtain multicomponent MOF derivatives by treating multicomponent MOFs under a suitable gas atmosphere and at high temperature. We used ZIF-67 as a template to introduce Zn and successfully obtained multicomponent MOFs. After carbonization, the multicomponent MOF derivatives with Co and CoO nanoparticles exhibit higher conversion of styrene (approximate to 99%), higher selectivity (approximate to 70%) and better stability compared to MOFs and single component MOF derivatives.
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