Journal
NANOSCALE
Volume 5, Issue 13, Pages 6097-6105Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3nr00988b
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Funding
- European Union [228762]
- Apulia Regional Projects RELA-VALBIOR POR FSE
- Laboratorio Regionale di Sintesi e Caratterizzazione di Nuovi Materiali Organici e Nanostrutturati per Elettronica, Fotonica e Tecnologie Avanzate
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A flexible host has been selected to achieve, for the first time, functional nanocomposites based on CdSe@ZnS core-shell type quantum dots (QDs) and Au nanoparticles (NPs), simultaneously dispersed in a polymer matrix. Coherent interactions between QDs and plasmonic Au NPs embedded in PDMS films have been demonstrated to lead to a relevant enhancement of the absorption cross-section of the QDs, remarkably modifying the optical response of the entire system. Optical and time resolved spectroscopy studies revealed an active gain-plasmon feedback behind the super-absorbing overall effect.
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