Article
Chemistry, Physical
Xiuhong Sun, Zhipeng Shao, Zhipeng Li, Dachang Liu, Caiyun Gao, Chen Chen, Bingqian Zhang, Lianzheng Hao, Qiangqiang Zhao, Yimeng Li, Xianzhao Wang, Yue Lu, Xiao Wang, Guanglei Cui, Shuping Pang
Summary: In this study, the open-circuit voltage of Cs-based perovskite solar cells was significantly enhanced by constructing a CsPbI3/Cs(1-x)DMA(x)PbI(3) bulk heterojunction structure, leading to improved charge separation and collection efficiency as well as reduced carrier recombination loss. This research suggests that junction engineering could be a new strategy for efficient perovskite devices.
Article
Chemistry, Physical
Xiaoxu Huang, Rongbin Xie, Hisashi Sugime, Suguru Noda
Summary: The performance of carbon nanotube/silicon solar cells was significantly improved by applying solution-processable MoOx, leading to a 39% increase in power conversion efficiencies. The MoOx acts as an efficient chemical dopant and an anti-reflection coating, reducing series resistance and enhancing short-circuit current density of the cell.
APPLIED SURFACE SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Stefan W. Tabernig, Lin Yuan, Andrea Cordaro, Zhi Li Teh, Yijun Gao, Robert J. Patterson, Andreas Pusch, Shujuan Huang, Albert Polman
Summary: We have designed an optically resonant bulk heterojunction solar cell to study the optoelectronic properties of nanostructured p-n junctions. By optimizing the nanoscale pattern, we were able to improve the efficiency of the solar cell by enhancing the absorption and charge-carrier extraction behavior. Our experiments and simulations showed significant improvement in infrared response and current gain in the patterned solar cell compared to the planar reference, demonstrating the importance of nanostructured geometries in enhancing solar cell performance.
Article
Chemistry, Physical
Yuan Xu, Guodong Li, Ruoshui Li, Yu Jing, Huayan Zhang, Xin Wang, Zhenbo Du, Jihuai Wu, Zhang Lan
Summary: In this study, a PbS/CdS heterojunction thin layer was constructed through interface engineering, which successfully improved the stability and efficiency of carbon-based CsPbI1.5Br1.5 solar cells.
Article
Chemistry, Analytical
Fei Zhao, Seth L. Filbrun, Tengxiang Huang, Bin Dong, Ning Fang
Summary: A multimodality spectromicroscopy imaging system has been developed to characterize functional materials under external stimuli, revealing the impact of thermal stress on the performance of the photoactive layer in bulk heterojunction solar cells. Continuous monitoring of the thermotropic evolution stages identified optimized thermal annealing temperature and preferred temperature dropping operation to enhance the photoactive layer performance.
ANALYTICAL CHEMISTRY
(2021)
Article
Chemistry, Multidisciplinary
Gideon Oyibo, Thomas Barrett, Sharadh Jois, Jeffrey L. Blackburn, Ji Ung Lee
Summary: This study presents an all-semiconducting single-walled carbon nanotube device with a tandem geometry that models the process of photosynthesis. By separating the light absorption and power generation processes using distinct chirality and bandgap single-walled carbon nanotubes, the device captures photons from multiple regions of the solar spectrum and enhances the photoresponse.
Article
Chemistry, Multidisciplinary
Ling Hong, Huifeng Yao, Yong Cui, Pengqing Bi, Tao Zhang, Yongxin Cheng, Yunfei Zu, Jinzhao Qin, Runnan Yu, Ziyi Ge, Jianhui Hou
Summary: Establishing an ideal architecture with selective carrier transport and suppressed recombination is crucial for improving photovoltaic efficiency in organic solar cells (OSCs). By tailoring a hybrid planar/bulk structure, highly efficient OSCs with reduced energy losses were fabricated. The study highlights the potential of precisely regulating the structure of donor:acceptor heterojunction to further enhance the efficiencies of OSCs.
ADVANCED MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Yeongkwon Kang, Jung Won Yoon, Seok Woo Lee, Hyungju Ahn, Siwon Yun, Jongchul Lim, Jihoon Lee, Dong Wook Chang, Hyosung Choi, Bong-Gi Kim
Summary: To investigate the effect of miscibility between conjugated polymers (CPs) and Y6 on the morphology of bulk-heterojunction (BHJ) structures, three different CPs with similar chemical structures but varying miscibility with Y6 were studied. The interface morphology and interlocked dimensions were compared quantitatively using a square-wave model after selectively removing Y6 from the CP/Y6 blend films. It was found that as CP-Y6 miscibility increases, a higher intermixed interface is formed, while a decrease in miscibility leads to a decrease in the dimensions formed by phase separation and an increase in width.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Energy & Fuels
Tongfa Liu, Yu Li, Rongguo Xu, Lingyun Lou, Jinqiang Gao, Kai Zhang, Mingzhu Su, Wei Qian, Gaopeng Wang, Shuang Xiao, Shihe Yang
Summary: An innovative perovskite/carbon bulk heterojunction for carbon-based perovskite solar cells is developed and studied, leading to improved efficiency and stability of the cells.
Article
Chemistry, Multidisciplinary
Wenwen Shi, Dongfeng Li, Dandan Tu, Deng Li, Wei Yu, Jingying Shi, Can Li
Summary: To overcome the poor stability of bulk heterojunction (BHJ) based photoelectrodes in aqueous environment, researchers have developed an inside and outside integrated modification method. The BHJ (PBDB-T:ITIC:PC71BM)-based photocathode with surface carbon protective layer showed sustained and fast photoelectrochemical (PEC) hydrogen evolution with an average photocurrent density of up to 13.5 mA cm(-2) for a duration of 15 hours.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Analytical
Sopan M. Wagalgave, Avinash C. Mendhe, Dinesh N. Nadimetla, Mohammad Al Kobaisi, Babasaheb R. Sankapal, Sidhanath Bhosale, Sheshanath Bhosale
Summary: Two DPP derivatives, DPP1 and DPP2, were synthesized with phenyl and thiophene moieties, respectively. DPP2 showed enhanced emissive properties and higher power conversion efficiency in dye sensitized solar cells compared to DPP1, likely due to differences in their photophysical and electrochemical properties.
JOURNAL OF ELECTROANALYTICAL CHEMISTRY
(2021)
Article
Materials Science, Multidisciplinary
Dhanasekaran Vikraman, Sajjad Hussain, Hailiang Liu, Syed Hassan Abbas Jaffery, K. Karuppasamy, Jun-Ho Lee, A. Kathalingam, Jongwan Jung, Hyun-Seok Kim
Summary: This paper introduces a facile solution route to fabricate MoTe2 grain nano-domains for hybrid polymer heterojunction solar cells and photodetectors. The effects of different MoTe2 nanostructure proportions on the performance of solar cells and photodetectors were investigated. Maximum power conversion efficiency of 8.94% was achieved for solar cells with 10 vol% MoTe2 nanostructure inclusion. A fabricated photodetector using 10 vol%-MoTe2 @PBDB-T:ITIC film achieved maximum detectivity of 2.62 x 10(10) Jones under 656 nm laser source.
JOURNAL OF MATERIALS RESEARCH AND TECHNOLOGY-JMR&T
(2022)
Article
Optics
Daniel A. Fentahun, Alekha Tyagi, Kamal K. Kar
Summary: The study found that the power conversion efficiency of AZO/Cu2O-based heterojunction thin-film solar cells is enhanced by using a double buffer (ZnO/CdS) layer compared to a single buffer (CdS) layer. The optimized solar cell structure with double buffer layers showed better performance under illumination.
Article
Chemistry, Multidisciplinary
Xian-Gang Hu, Yi-Ming Zhao, Hongyu Yang, Peng-Xiang Hou, Chang Liu, Jingjing Chang, Yue Hao
Summary: A multifunctional Lewis acid, p-toluenesulfonic acid (TsOH), is used to optimize and tune the properties of single-wall carbon nanotube/silicon (SWCNT/Si) solar cells. TsOH acts as a charge transfer doping agent, optimizing the conductivity and work function of SWCNT films. Additionally, a chemical bridge is formed at the interface of SWCNT/Si heterojunction, effectively suppressing carrier recombination and enhancing the photocurrent. The TsOH coating also functions as an antireflection layer, leading to an increase in the power conversion efficiency.
Article
Materials Science, Multidisciplinary
Jun Zan, Yujuan Huang, Huiqin Cui, Jianbin Chen, Longlong Zhang
Summary: In donor-acceptor (D-A) heterojunction polymer solar cells, photocreated excitons evolve into the charge-transfer (CT) state at D/A interfaces. In some cases, the exciton can also trap one charge by forming a trion state. The mechanisms of charge transfer and separation for these trions at D/A interfaces are still not fully understood but they are crucial for photovoltaic performance. In this study, the electronic properties of the trion-CT state were theoretically investigated using a tight-binding model. The results show that the interfacial trion-CT state remains a bound state with one electron transferring to the acceptor and one exciton remaining on the donor. The amount of charge transfer can be adjusted by intrinsic factors including charge delocalization, D-A coupling strength, electron-lattice and electron-electron interactions, and the D-A energetic offset. Charge separation of the trion-CT state under an electric field was also studied, and the results suggest that the trion-CT state is harder to dissociate compared to the exciton-CT state.
ORGANIC ELECTRONICS
(2023)
Article
Psychology, Multidisciplinary
Mike Lin, Fengxiang Zhang, Xiaomin Sun, Nan Zhang, Jiaqi Wang, Yanqiang Tao, Zhenzhen Liu
Summary: This research examines the relationship between procedural fairness and participation in development activities (PDA), the underlying mechanism, and the boundary condition of the relationship, drawing on attribution theory. The results show that procedural fairness positively predicts PDA, and self-attribution mediates their relationship. In addition, self-construal moderates the relationship between self-attribution and PDA.
CURRENT PSYCHOLOGY
(2023)
Review
Medicine, Research & Experimental
Siyi Lu, Zhaoyu Chen, Zhenzhen Liu, Zhentao Liu
Summary: NOC2L, a novel inhibitor of histone acetyltransferase (INHAT), regulates histone acetylation in a HDAC-independent manner and has two INHAT function domains. This review summarizes the biological function of NOC2L in histone acetylation regulation, P53-mediated transcription, ribosome RNA processing, certain development events, and carcinogenesis. NOC2L may serve as a potential biomarker and therapeutic target in clinical practice.
JOURNAL OF TRANSLATIONAL MEDICINE
(2023)
Article
Chemistry, Physical
Yanfang Ding, Huanhuan Sun, Zhihao Li, Chunmei Jia, Xiaogang Ding, Can Li, Jian-Gan Wang, Zhen Li
Summary: A simple and scalable galvanic-driven strategy was used to deposit large-area Prussian Blue (PB) films on both rigid and flexible substrates. A flexible PB/Zn battery-type electrochromic device with multiple functions was constructed, including a flexible power source and capacity depletion visualization. The device exhibited excellent properties with a large optical contrast, high coloration efficiency, rapid switching, long-operation stability, and good flexibility, making it a promising flexible power source for real-world applications.
JOURNAL OF MATERIALS CHEMISTRY A
(2023)
Article
Agronomy
Zhendong Liu, Shiyu Wei, Ming Li, Qingfen Zhang, Rui Zong, Quanqi Li
Summary: This study examined the effects of planting density and genotypes on the leaf area index, photosynthetic characteristics, dry-matter accumulation, water-use efficiency, and yield of summer maize. Increasing planting density enhanced light interception and dry-matter accumulation but decreased chlorophyll content, net photosynthetic rate, and transpiration rate. Both high and low planting densities were detrimental to yield and resource-use efficiency. Denghai 605 showed a higher yield potential and water-use efficiency compared to Zhengdan 958.
Article
Medicine, General & Internal
Chunmei Jiang, Zhixiang Xu, Jin Li, Jiaqi Zhang, Xingkui Xue, Jingxia Jiang, Guihua Jiang, Xisheng Wang, Yun Peng, Tian Chen, Zhenzhen Liu, Liu Xie, Haibin Gao, Yingxia Liu, Yang Yang
Summary: In this case study, a 31-year-old immunocompetent adult was diagnosed with aseptic meningitis caused by recombinant echovirus 18. The patient recovered after 4 days of antiviral treatment. This is the first report of echovirus 18-induced meningitis in an immunocompetent adult from mainland China, highlighting the importance of surveillance for echovirus 18 infection in both children and adults.
FRONTIERS IN MEDICINE
(2023)
Article
Biochemistry & Molecular Biology
Yuyin Li, Yaxin Zhang, Lu Li, Mei Zhang, Ning Song, Qing Zhao, Zhenxing Liu, Aipo Diao
Summary: The transmembrane prostate androgen-induced protein (TMEPAI) is highly expressed in various types of cancer and activates the NF-kappa B signaling pathway through the ubiquitination of I kappa B alpha. This results in the degradation of I kappa B alpha and the subsequent activation of NF-kappa B signaling. Further investigation revealed that TMEPAI-induced cell proliferation and tumor growth in immune deficient mice are mediated by the NF-kappa B signaling pathway. This study provides valuable insights into the role of TMEPAI in tumorigenesis and suggests it as a potential target for cancer treatment.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2023)
Article
Biochemistry & Molecular Biology
Ke Ma, Wei Chen, Xiao-Qi Lin, Zhen-Zhen Liu, Tao Wang, Jia-Bao Zhang, Jian-Gang Zhang, Cheng-Kai Zhou, Yu Gao, Chong-Tao Du, Yong-Jun Yang
Summary: Pure cultures of chicken intestinal microbial species are important for understanding gut microbiota function and developing potential probiotics and bioactive metabolites. This study isolated and identified 507 bacterial isolates, including 89 previously uncultured ones, with 63 Lactobacillus strains exhibiting antibacterial activity against S. Pullorum. L. reuteri strain YPG14 showed strong acid tolerance and other probiotic properties, and its consumption significantly improved body weight, reduced S. Pullorum loads, and alleviated damage caused by S. Pullorum.
INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES
(2023)
Article
Microbiology
Ting-Ting Du, Xiao-Chen Liu, Yu He, Xiong Gao, Zhen-Zhen Liu, Zheng-Li Wang, Lu-Quan Li
Summary: This study aimed to explore the value of gut microbiota and tricarboxylic acid (TCA) metabolites in early diagnosis of NEC among infants with abdominal manifestations. High-throughput sequencing was used to analyze the gut microbiota, and multiple reaction monitoring (MRM) targeted metabolomics was used to measure TCA metabolites. The results showed that decreased levels of unclassified Staphylococcus, Lactobacillaceae, and Bifidobacterium animalis subsp. lactis at the species level, as well as increased levels of succinate, L-malic acid, and oxaloacetate, have potential value for the early diagnosis of NEC.
FRONTIERS IN MICROBIOLOGY
(2023)
Article
Chemistry, Physical
Chongyang Zhi, Suo Wang, Shijing Sun, Can Li, Zhihao Li, Zhi Wan, Hongqiang Wang, Zhen Li, Zhe Liu
Summary: Interface passivation using an ammonium salt improves the power conversion efficiency of perovskite solar cells. A machine-learning method is used to investigate the relationship between the molecular features of ammonium salts and the efficiency improvement. Hydrogen bond donor, hydrogen atom, and octane-water partition coefficient are identified as important features for selecting an ammonium salt. The ML model is used to screen salts and achieves high PCEs for FAMACs and FAMA-based PSCs.
ACS ENERGY LETTERS
(2023)
Article
Pharmacology & Pharmacy
Hua Miao, Yan-Ni Wang, Xiao-Yong Yu, Liang Zou, Yan Guo, Wei Su, Fei Liu, Gang Cao, Ying-Yong Zhao
Summary: This study identified alterations in gut microbiota and serum metabolites mediating an AhR mechanism in MN rats and IMN patients, providing insights into the pathogenesis of MN.
BRITISH JOURNAL OF PHARMACOLOGY
(2023)
Article
Chemistry, Physical
Weixue Meng, Jing Wang, Ding Zhang, Jie Xu, Fengmei Guo, Yingjiu Zhang, Rui Pang, Anyuan Cao, Yuanyuan Shang
Summary: Compared to HER under acidic conditions, alkaline HER involves more complex kinetic steps, including the adsorption and cleavage of water molecules. Defect and interface engineering are important methods to enhance alkaline HER. In this study, a catalyst composed of a defective amorphous carbon loaded with Ru nanoparticles wrapped around a carbon nanotube sponge network was prepared. The presence of amorphous carbon promotes uniform loading and limits the growth of Ru nanoparticles, while the introduction of oxygen defects improves charge transport capacity and catalytic performance. The optimized catalyst exhibited excellent stability and activity, with low overpotentials under both alkaline and acidic conditions, surpassing most reported Ru-based catalysts. These findings provide innovative and feasible ideas for the design and preparation of loaded catalysts, contributing to the development of high-performance electrochemical catalysts.
Article
Chemistry, Multidisciplinary
Zhanchen Guo, Qi Zhang, Rongrong Xing, Zhen Liu
Summary: Using two molecularly imprinted and cladded polymers, researchers developed an inexpensive, fast, and portable plasmonic immuno-sandwich assay for highly specific and ultra-sensitive detection of C-peptide in urine. This method, based on dual cMIPs, showed promising potential in clinical diagnosis by distinguishing healthy individuals from diabetes patients and exhibiting significant advantages over existing immunoassays.
CHEMICAL COMMUNICATIONS
(2023)
Article
Chemistry, Multidisciplinary
Pengfei Li, Shuxin Xu, Yanjie Han, Hui He, Zhen Liu
Summary: A machine learning-empowered mass spectrometry platform was developed for accurate profiling and quantification of cis-diol metabolites associated with liver cancer. The platform improved the detection coverage and demonstrated higher sensitivity and specificity in diagnosing liver cancer compared to protein biomarker-based methods.
Article
Chemistry, Physical
Liangzheng Dong, Shengye Tao, Ming Zhao, Daming Zhuang, Yafei Wang, Hanpeng Wang, Mengyao Jia, Junsu Han, Hongwei Zhu
Summary: Alkali metal doping in Cu2ZnSn(S,Se)(4) (CZTSSe) thin film solar cells has been found to promote the crystallization process and improve the electrical properties of the grain boundaries and heterojunction band alignments. The K-doped CZTSSe solar cells exhibit better device performance and fewer defects.
JOURNAL OF MATERIALS CHEMISTRY A
(2023)
Article
Chemistry, Physical
Meirong Huang, Sutong Wang, Hongwei Zhu
Summary: In this study, a comprehensive machine learning process was introduced to guide the selection of cocatalysts for BiVO4 photoanodes. The models trained using neural network and ensemble techniques were able to capture intricate relationships among photoanodes, cocatalysts, and electrolytes, and accurately predict unstudied cases. The feature importance analysis revealed that the type and preparation method of cocatalysts were the most significant factors affecting the catalytic system's performance. The interpretability of the models provided heuristic rules for selecting promising cocatalysts for BiVO4 photoanodes.
JOURNAL OF MATERIALS CHEMISTRY A
(2023)