4.8 Article

Quantum Hall Effect in Electron-Doped Black Phosphorus Field-Effect Transistors

Journal

NANO LETTERS
Volume 18, Issue 10, Pages 6611-6616

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.8b03267

Keywords

Black phosphorus; field-effect transistor; two-dimensional electron gas; quantum Hall effect; electron-electron interaction

Funding

  1. National Science Foundation [DMR-1157490, DMR-1644779]
  2. State of Florida
  3. National Key Research Program of China [2016YFA0300703, 2018YFA0305600]
  4. NSF of China [U1732274, 11527805, 11425415, 11421404, 11604053, 11434010]
  5. Strategic Priority Research Program of Chinese Academy of Sciences [XDB30000000]
  6. China Postdoctoral Science Foundation [2016M600279, 2017T100264]
  7. Strategic Priority Research Program of the Chinese Academy of Sciences [XDB04040100]
  8. National Basic Research Program of China (973 Program) [2012CB922002]
  9. National Natural Science Foundation of China [11534010]
  10. Key Research Program of Frontier Sciences, CAS [QYZDY-SSW-SLH021]
  11. MEXT, Japan
  12. JSPS KAKENHI [JP15K21722]

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The advent of black phosphorus field-effect transistors (FETs) has brought new possibilities in the study of two-dimensional (2D) electron systems. In a black phosphorus FET, the gate induces highly anisotropic 2D electron and hole gases. Although the 2D hole gas in black phosphorus has reached high carrier mobilities that led to the observation of the integer quantum Hall effect, the improvement in the sample quality of the 2D electron gas (2DEG) has however been only moderate; quantum Hall effect remained elusive. Here, we obtain high quality black phosphorus 2DEG by defining the 2DEG region with a prepatterned graphite local gate. The graphite local gate screens the impurity potential in the 2DEG. More importantly, it electrostatically defines the edge of the 2DEG, which facilitates the formation of well-defined edge channels in the quantum Hall regime. The improvements enable us to observe precisely quantized Hall plateaus in electron-doped black phosphorus FET. Magneto-transport measurements under high magnetic fields further revealed a large effective mass and an enhanced Lande g-factor, which points to strong electron-electron interaction in black phosphorus 2DEG. Such strong interaction may lead to exotic many-body quantum states in the fractional quantum Hall regime.

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