4.8 Article

Spin-Orbit Interaction in a Two-Dimensional Hole Gas at the Surface of Hydrogenated Diamond

Journal

NANO LETTERS
Volume 15, Issue 1, Pages 16-20

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nl502081y

Keywords

Diamond; surface conductivity; spin-orbit interaction; 2DHG

Funding

  1. Australian Research Council [DP0879827]
  2. Australian Nanotechnology Network, Department of Innovation, Industry, Science and Research
  3. Australian Synchrotron
  4. Australian Research Council [DP0879827] Funding Source: Australian Research Council

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Hydrogenated diamond possesses a unique surface conductivity as a result of transfer doping by surface acceptors. Yet, despite being extensively studied for the past two decades, little is known about the system at low temperature, particularly whether a two-dimensional hole gas forms at the diamond surface. Here we report that (100) diamond, when functionalized with hydrogen, supports a p-type spin-3/2 two-dimensional surface conductivity with a spinorbit interaction of 9.74 +/- 0.1 meV through the observation of weak antilocalization effects in magneto-conductivity measurements at low temperature. Fits to 2D localization theory yield a spin relaxation length of 30 +/- 1 nm and a spin-relaxation time of similar to 0.67 +/- 0.02 ps. The existence of a 2D system with spin orbit coupling at the surface of a wide band gap insulating material has great potential for future applications in ferromagnetsemiconductor and superconductorsemiconductor devices.

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