4.8 Article

Self-Assembled ErSb Nanostructures with Optical Applications in Infrared and Terahertz

Journal

NANO LETTERS
Volume 14, Issue 3, Pages 1107-1112

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nl402436g

Keywords

Self-assembly; nanostructures; surface plasmon; optical polarization; terahertz; molecular beam epitaxy

Funding

  1. Worster Fellowship at UCSB
  2. Defense Advanced Research Projects Agency Nanostructured Materials for Power program
  3. Center for Energy Efficient Materials, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001009]
  4. Humboldt foundation
  5. NSF MRSEC program [DMR-0520415]
  6. Division Of Materials Research
  7. Direct For Mathematical & Physical Scien [1006603] Funding Source: National Science Foundation

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Plasmonic effects have proven to be very efficient in coupling light to structures much smaller than its wavelength. Efficient coupling is particularly important for the infrared or terahertz (lambda similar to 0.3 mm) region where semiconductor structures and devices may be orders of magnitude smaller than the wavelength and this can be achieved through nanostructures that have a desired plasmonic response. We report and demonstrate a self-assembly method of embedding controllable semimetallic nanostructures in a semiconducting matrix in a ErSb/GaSb material system grown by molecular beam epitaxy. The plasmonic properties of the ErSb/GaSb are characterized and quantified by three polarization-resolved spectroscopy techniques, spanning more than 3 orders of magnitude in frequency from 100 GHz up to 300 THz. Surface plasmons cause the semimetallic nanostructures to resonate near 100 THz (3 mu m wavelength), indicating the semimetal as a potential infrared plasmonic material. The highly conductive ErSb nanowires polarize electromagnetic radiation in a broad range from 0.2 up to similar to 100 THz, providing a new platform for electromagnetics in the infrared and terahertz frequency ranges

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