Journal
NANO LETTERS
Volume 10, Issue 8, Pages 2761-2765Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nl100253r
Keywords
Nanocrystal; fluorescence intermittency; memory effect; long-range dependence; single molecule; nanowire
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Funding
- Institute for Theoretical Sciences, the Department of Energy, Basic Energy Sciences
- National Science Foundation via the NSF-NIRT [ECS-0609249]
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We explain the long-range correlations found by Stefani and his co-workers between blinking times of single colloidal quantum dot emission. Our explanation is based on the multiple recombination center model we recently suggested. The model produces positive correlations between subsequent-on on and off-off times and negative on-off correlations, as observed in the experiment. we also reproduce qualitatively the dependence of correlations between subsequent on-on, on-off, and off-off times on the number of switching events separating them.
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