Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 136, Issue 11, Pages 4097-4100Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja411433f
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Funding
- National Science Foundation [CHE-1111563, CHE-0840456]
- Foundation Ramon Areces Fellowship
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1111563] Funding Source: National Science Foundation
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This communication describes the design of a model system that allows direct investigation of competing sp(3)-C-N and sp(3)-C-F bond-forming reductive elimination from a Pd-IV fluoro sulfonamide complex. The reductive elimination selectivity varies dramatically as a function of reaction additives. A mechanism is proposed that provides a rationale for these effects.
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