Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 3, Pages 971-974Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja3110818
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Funding
- National Natural Science Foundation of China [20972172, 21021063]
- Chinese Academy of Sciences
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New, simple, sulfinamide-based branched olefin ligands have been developed and successfully used in Rh-catalyzed asymmetric arylations of cyclic ketimines, providing efficient and highly enantioselective access to valuable benzosultams and benzosulfamidates containing a stereogenic quaternary carbon center. This is the first example of applying a sulfur-olefin ligand in catalytic asymmetric addition of imines.
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