Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 12, Pages 4696-4699Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja401380d
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Funding
- NSF [CAREER 0643264]
- American Cancer Society [RSG-09-017-01-CDD]
- NSF
- Abbott
- Eli Lilly
- Roche
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Rh-bound trimethylenemethane variants generated from the interaction of a Rh-carbenoid with an allene have been applied to the synthesis of substituted 3,4-fused pyrroles. The pyrrole products are useful starting points for the syntheses of various dipyrromethene ligands. Furthermore, the methodology has been applied to a synthesis of the natural product cycloprodigiosin, which demonstrates antitumor and immunosuppressor activity.
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