Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 13, Pages 4992-4995Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja401936c
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Funding
- EPSRC [EP/G036764/1]
- Syngenta
- Royal Society
- EPSRC [EP/K03927X/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [981180, EP/K03927X/1] Funding Source: researchfish
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Aminocyclopropanes equipped with suitable N-directing groups undergo efficient and regioselective Rh-catalyzed carbonylative C-C bond activation. Trapping of the resultant metallacycles with tethered alkynes provides an atom-economic entry to diverse N-heterobicyclic enones. These studies provide a blueprint for myriad N-heterocyclic methodologies.
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