Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 30, Pages 10974-10977Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja405581r
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Funding
- NSF [CHE-1112278]
- Medtronic Inc.
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Polyketals are an important class of materials for drug delivery to sensitive tissues as they degrade in vivo to nonacidic species. We report the synthesis of high-molecular weight cyclic polyketals by the cationic ring-opening polymerization of bicyclic ketal monomers, which were prepared by the metal-catalyzed rearrangement of epoxy ketones. Three different cyclic polyketals with high molecular weights were synthesized using this protocol.
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