Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 29, Pages 11995-11997Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja305856q
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Funding
- Japan Society for the Promotion of Science (JSPS) [20002004, 22590002]
- Research Foundation for Pharmaceutical Sciences
- Mochida Memorial Foundation for Medical and Pharmaceutical Research
- Uehara Memorial Foundation
- Grants-in-Aid for Scientific Research [22590002, 20002004] Funding Source: KAKEN
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A first asymmetric total synthesis of (-)-isoschizogamine has been accomplished. Our synthesis features the facile construction of the carbon framework of the natural product through a Wagner-Meerwein rearrangement, a tandem metathesis, a stereo-selective rhodium-mediated 1,4-addition of an arylboronic acid, and a ring-closing metathesis via a hemiaminal ether.
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