Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 133, Issue 6, Pages 1690-1693Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja110039h
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Funding
- Natural Science Foundation of China [20825205, 21072013]
- National Basic Research Program of China (973 Programs) [2011CB808600, 2010CB833203]
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A novel Rh(I)-catalyzed formal [5 + 1]/[2 + 2 + 1] cycloaddition of 1-yne-vinylcydopropanes and two CO units for the construction of multifunctional angular tricyclic 5/5/6 skeletons with one or two adjacent bridgehead quaternary all-carbon stereocenters in one step has been developed. Preliminary density functional theory calculations have been carried out to investigate the reaction mechanism and the substituent effects.
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