Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 132, Issue 36, Pages 12550-12551Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja1058247
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- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC-0001298]
- DOE [DE-FG02-84ER13297]
- U.S. Department of Energy (DOE) [DE-FG02-84ER13297] Funding Source: U.S. Department of Energy (DOE)
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A series of (CpIr)-Ir-star complexes can catalyze C-H oxidation, with ceric ammonium nitrate as the terminal oxidant and water as the source of oxygen. Remarkably the hydroxylation of cis-decalin and 1,4-dimethylcyclohexane proceeds with retention of stereochemistry. With H2O18, cis-decalin oxidation gave O-18 incorporation into the product cis-decalol.
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