Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 131, Issue 2, Pages 585-589Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja806211r
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The structure of the carbon dioxide-water interface was analyzed by X-ray diffraction and reflectivity at temperature and pressure conditions which allow the formation of gas hydrate. The water-gaseous CO(2) and the water-liquid CO(2) interface were examined. The two interfaces show a very different behavior with respect to the formation of gas hydrate. While the liquid-gas interface exhibits the formation of thin liquid CO(2) layers on the water surface, the formation of small clusters of gas hydrate was observed at the liquid-liquid interface. The data obtained from both interfaces points to a gas hydrate formation process which may be explained by the so-called local structuring hypothesis.
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