Article
Engineering, Environmental
Kajal Sharma, Ravinder Kaushik, Pawan Kumar Pandey, Sumanta Chowdhury, Rituporn Gogoi, Astha Singh, Aditi Halder, Prem Felix Siril
Summary: In this study, hierarchical and hollow microspheres assembly of one-dimensional zinc-trimesic acid (Zn-BTC) MOF nanospikes were successfully synthesized using a single step solvothermal synthesis method. The formed Zn-BTC hierarchical and hollow microspheres were annealed to form ZnO/C hierarchical nanocomposite microspheres. These hierarchical nanocomposite microspheres exhibited enhanced photocatalytic activities for water remediation. The improved photocatalytic performance was attributed to the synergistic effect between the carbon matrix and well-dispersed ZnO quantum dots.
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
(2022)
Article
Nanoscience & Nanotechnology
Dong Seob Chung, Tyler Davidson-Hall, Giovanni Cotella, Quan Lyu, Peter Chun, Hany Aziz
Summary: This study shows that incorporating fluorine into ZnO ETLs can significantly enhance the electroluminescence stability of QLEDs, leading to an extended device lifetime by balancing electron and hole distribution and reducing electron traps and charge accumulation at the QD/hole transport layer interface.
NANO-MICRO LETTERS
(2022)
Article
Engineering, Environmental
Walied A. A. Mohamed, Hala T. Handal, Ibrahem A. Ibrahem, Hoda R. Galal, Hanan A. Mousa, Ammar A. Labib
Summary: The solar photocatalytic activity of zinc oxide quantum dots was investigated, with the first sample showing better performance in degradation rate of synthetic dye and higher efficiency in photo-oxidation compared to the second sample. The study also included an evaluation of mineralization and recycling efficiency of industrial wastewater with different doses of ZOQDs under sunlight for a year, meeting local environmental regulations.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Environmental Sciences
Huihui Feng, Yan Zhang, Fengling Cui
Summary: Cuprous oxide (Cu2O), a p-type semiconductor material, has been found to play a significant role in photocatalysis, and enhancing its photocatalytic activity can be effectively achieved by introducing CQDs, leading to improved degradation of methylene blue and antibacterial activity against Escherichia coli.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2022)
Article
Chemistry, Inorganic & Nuclear
Sumathi Subramanian, Sasikala Ganapathy, Suguna Subramanian, Ayyaswamy Arivarasan
Summary: A one-step approach is developed for the decoration of CdTe QDs onto the surface of GO nanosheets/integration of QDs into GO nanosheets through self-assembly, forming sandwiched hybrid heterojunctions. Interlinking QDs and GO nanosheets improves photocurrent generation (~5.8 μA cm-2) and enhances electron transfer by prolonging decay time (58.25 ms). The obtained higher rate constant value (k = 0.135 min-1) enables the degradation of 93% MB dye in 20 min. This work demonstrates a cost-effective strategy for constructing CdTe QDs/GO nanosheet hybrid heterojunctions with potential application in photocatalysis.
DALTON TRANSACTIONS
(2023)
Article
Chemistry, Physical
Tingting Cai, Qing Chang, Bin Liu, Caihong Hao, Jinlong Yang, Shengliang Hu
Summary: A carbon dot-based composite (CDs@CuOx) is introduced to eliminate charge accumulation and boost photocatalytic activity through triggering a chemical reaction. The chemical conversion rapidly consumes photoinduced electrons and holes, eliminating surface polarization and significantly enhancing photocatalytic activity.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Article
Environmental Sciences
Ali Reza Amani-Ghadim, Samira Arefi-Oskoui, Robab Mahmoudi, Abdolreza Tarighati Sareshkeh, Alireza Khataee, Fatemeh Khodam, Mir Saeed Seyed Dorraji
Summary: Inserting Gd ions into the crystalline lattice of ZnS quantum dots (QDs) enhanced their photo-catalytic activity. The influence of graphene oxide (GO) and graphitic carbon nitride (g-C3N4) on the photocatalytic activity of the ZnS QDs was also investigated. The results showed that the presence of Gd-doped ZnS QDs/g-C3N4 nanocomposite achieved the highest photocatalytic degradation efficiency and total organic carbon removal.
Article
Physics, Multidisciplinary
Sarika Singh, Kamakhya Prakash Misra, Alveera Sohel, Rama Sharma
Summary: The objective of this study is to analyze the impact of shape and size alterations on the photoluminescence (PL) emission and photocatalytic activity of ZnO nanostructures. The study describes the controlled synthesis of ZnO nanoassemblies (NA) and nanocrystals (NC) using a soft chemical approach. The synthesized ZnO nanostructures were characterized using various techniques, including TEM, SEM, UV-vis, and PL measurement. The results show that the morphology of ZnO can be tuned by adjusting the molar ratio of DEG and water, which also affects the PL emission spectra. The controlled nanostructured growth demonstrates potential for sustainable photocatalytic activity under both UV and sunlight irradiation.
Article
Engineering, Electrical & Electronic
Tongtong Zhang, Qi Yin, Menghan Zhang, Siyu Zhang, Yanning Shao, Liyu Fang, Qishe Yan, Ximeng Sun
Summary: The composite heterojunction photocatalysts of reduced graphene (rGO) and AgBr show improved optical properties, higher degradation rate of Rhodamine B (RhB), and enhanced separation of photogenerated electrons and holes. The addition of graphene significantly promotes the photocatalytic degradation performance of the catalyst.
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
(2021)
Article
Engineering, Environmental
Lijiao Ao, Tao Liao, Liang Huang, Shan Lin, Kui Xu, Jiangtao Ma, Shaorong Qiu, Xiangyu Wang, Qiqing Zhang
Summary: This study developed a highly sensitive and portable multi-target serum cancer biomarker detection method. By using NIR-II emitting quantum dots and three-dimensional distribution assembly, the sensitivity and fluorescence signals of the test strip were successfully enhanced. With this method, simultaneous detection and quantitative analysis of CEA, Cyfra21-1, and NSE tumor biomarkers were achieved, with high sensitivity and specificity demonstrated in lung cancer patients and healthy individuals.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Multidisciplinary
Emel Kirbas Cilingir, Meghana Sankaran, Jordan M. Garber, Frederic Anthony Vallejo, Mattia Bartoli, Alberto Tagliaferro, Steven Vanni, Regina M. Graham, Roger M. Leblanc
Summary: Carbon dots (CDs) have gained attention for their biocompatibility and tunable photoluminescence, but further analysis is needed before their use in clinical trials. A new type of carbon nitride dot (CND) has been found to selectively uptake cancer cells due to structural similarities with glutamine. The study investigates the effects of surface structural differences on the cellular uptake of CNDs and finds that the uptake mechanism is linked with ASCT2 and LAT1 transporters. CNDs show promise for selective cancer cell targeting by utilizing highly expressed transporters on cancer cells.
Article
Chemistry, Multidisciplinary
Agnieszka Fiszka Borzyszkowska, Agnieszka Sulowska, Pawel Czaja, Aleksandra Bielicka-Gieldon, Ivar Zekker, Anna Zielinska-Jurek
Summary: This study successfully synthesized multi-doped carbon dots (xCDs) with excellent fluorescence properties from microalga Chlorella pyrenoidosa using simple hydrothermal and microwave-assisted methods. The nonmetal doping in the nanomaterials was confirmed by XPS, while the existence of metals in the CDs was confirmed by ICP-OES and TEM, with Mg, Ca, K, and Na being the dominant doped metals. The synthesized xCDs were used for the modification of ZnO, and their photocatalytic properties were evaluated, showing promising potential for the degradation of carbamazepine.
Article
Chemistry, Inorganic & Nuclear
Nikhita Khurana, Pinklesh Arora, Avinash S. Pente, Keyur C. Pancholi, Virendra Kumar, Chetan P. Kaushik, Sunita Rattan
Summary: This article investigates the effect of different concentrations of vinyl triethoxysilane (VTES) on the surface modification of zinc oxide nanoparticles. Characterization techniques such as FTIR, TGA, SEM, EDX, XRD and contact angle confirm that a 15 wt% concentration of VTES is suitable for the surface modification of ZnO nanoparticles.
INORGANIC CHEMISTRY COMMUNICATIONS
(2021)
Article
Chemistry, Physical
Adil Alshoaibi, Shumaila Islam
Summary: Sol-gel-based titania nanoparticles, Silica-titania nanocomposite, and zinc supported silica-titania nanocomposites were synthesized at low temperature. The study showed that zinc nanoparticles were homogeneously distributed in the silica-titania nanocomposite, and the doping of zinc enhanced the photocatalytic activity of the material.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Chemistry, Multidisciplinary
Faxing Liu, Quanjun Xiang, Xigui Zhang, Haiping Zhou
Summary: In this study, Ni cocatalysts on a TiO2 composite photocatalyst with different graphene oxide (GO) contents were prepared using a hydrothermal method and characterized. It was found that the TiO2/GO/Ni nanosheet composites have a large specific surface area and can provide a large number of active sites for photocatalytic hydrogen production. GO can broaden the optical absorption range of TiO2 and absorb more visible light, stimulating the generation of more electron-hole pairs. Additionally, GO can collect electrons and promote the separation of electron-hole pairs. Ni, as a cocatalyst, can adsorb hydrogen ions and facilitate the migration of photogenerated electrons, thus ensuring high efficiency of the photocatalytic reaction.
NEW JOURNAL OF CHEMISTRY
(2023)
Review
Engineering, Chemical
Ankita Gagrani, Takuya Tsuzuki
CHEMICAL ENGINEERING SCIENCE
(2019)
Article
Chemistry, Physical
Jian Zhao, Wenjing Li, Linpeng Fan, Quan Quan, Jinfeng Wang, Changfa Xiao
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2019)
Review
Nanoscience & Nanotechnology
Esfandiar Pakdel, Maryam Naebe, Lu Sun, Xungai Wang
ACS APPLIED MATERIALS & INTERFACES
(2019)
Article
Chemistry, Physical
Zhenyu Li, Qiangbin Yang, Yuanpeng Wu, Yi He, Jingyu Chen, Jinfeng Wang
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2019)
Article
Polymer Science
Yujia Liang, Esfandiar Pakdel, Mingwen Zhang, Lu Sun, Xungai Wang
POLYMER DEGRADATION AND STABILITY
(2019)
Article
Polymer Science
Xinzhu Chen, Jing An, Guangming Cai, Jin Zhang, Wu Chen, Xiongwei Dong, Licheng Zhu, Bin Tang, Jinfeng Wang, Xungai Wang
Article
Materials Science, Multidisciplinary
Yujia Liang, Wanjie Xie, Esfandiar Pakdel, Mingwen Zhang, Lu Sun, Xungai Wang
MATERIALS CHEMISTRY AND PHYSICS
(2019)
Article
Chemistry, Multidisciplinary
Mazher Iqbal Mohammed, Daniel Wilson, Eli Gomez-Kervin, Bin Tang, Jinfeng Wang
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2019)
Article
Chemistry, Applied
Bin Tang, Ying He, Jun Liu, Jin Zhang, Jingliang Li, Ji Zhou, Yong Ye, Jinfeng Wang, Xungai Wang
Article
Green & Sustainable Science & Technology
Xi Lu, Zhenyu Li, Yu'an Liu, Bin Tang, Yanchao Zhu, Joselito M. Razal, Esfandiar Pakdel, Jinfeng Wang, Xungai Wang
JOURNAL OF CLEANER PRODUCTION
(2020)
Article
Polymer Science
Miaomiao Qian, Weimin Huang, Jinfeng Wang, Xiaofeng Wang, Weiping Liu, Yanchao Zhu
Article
Chemistry, Multidisciplinary
Ling Wang, Bin Tang, Ji Zhou, Hai Zhao, Wu Chen, Jinfeng Wang
APPLIED SCIENCES-BASEL
(2019)
Article
Chemistry, Multidisciplinary
Daiqi Li, Bin Tang, Xi Lu, Quanxiang Li, Wu Chen, Xiongwei Dong, Jinfeng Wang, Xungai Wang
APPLIED SCIENCES-BASEL
(2019)
Article
Materials Science, Multidisciplinary
Daiqi Li, Jinfeng Wang, Xi Lu, Wu Chen, Xiongwei Dong, Bin Tang, Xungai Wang
MATERIALS & DESIGN
(2019)
Article
Chemistry, Physical
Zhong Zhao, Chris Hurren, Mingwen Zhang, Liming Zhou, Jihong Wu, Lu Sun
Article
Materials Science, Ceramics
Zilong Xiong, Wenzhuo Xue, Mujun Li, Feihu Tan, Yupeng Chen, Hongyu Yu
Summary: In this study, CBS glass/Al2O3 composites were developed for LTCC applications based on a CaO-B2O3-SiO2 (CBS) glass system with a high boron content. The study revealed that the softening of glass and interfacial reaction between the glass and Al2O3 were the two most important factors affecting LTCC's densification process. Real-time shrinkage rate of LTCC during sintering was successfully simulated, and it was proven that the formation of the CaAl2(BO3)O phase played a significant role in reducing glass viscosity and promoting dense structure formation. The resulting LTCC composite exhibited excellent performance for high-frequency applications.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Saurabh Kumar Sharma, Vinita Grover, Rakesh Shukla, Abid Hussain, Ambuj Mishra, Pawan Kumar Kulriya
Summary: In this study, the disordering caused by swift heavy ion irradiation in two different compositions of pyrochlore structures was investigated. X-ray diffraction, Raman spectroscopy, and high-resolution transmission electron microscopy were used to analyze the samples before and after irradiation. It was found that both compositions underwent amorphization due to irradiation, with a slower rate observed in Nd1.8Zr2.2O7.1. The irradiation-induced modified track region in Nd1.8Zr2.2O7.1 consisted of defect-rich pyrochlore structure, anion-deficient fluorite structure, and amorphous domains.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Jiabei He, Mengshan Song, Ming Yang, Miaomiao Zhu
Summary: This study investigates the influence of ion irradiation on high-entropy ceramics and finds that irradiation-induced lattice rearrangement can improve the radiation resistance of these ceramics.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Yajie Yu, Shi He, Zhengang Zhang, Haihua Chen, Peipeng Jin, Binnian Zhong, Linhui Zhang, Liping Wang, Cheng Lu
Summary: Silicide ceramics, including tantalum disilicide (TaSi2), are known for their exceptional physical properties but are limited in practical applications due to their inherent brittleness at room temperature. In this study, we successfully improved the mechanical properties of TaSi2 ceramics and increased their electrical conductivity by modifying the preparation methods and sintering conditions. These findings provide valuable insights for future applications of TaSi2 and the design of advanced ceramic materials.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Jian Li, Jia Liu, Yongcui Zhang, Wei Sun, Yang Wang, Haitao Wu, Ling Li, Chuanbing Cheng, Yingying Wang, Ke Tan, Futian Liu
Summary: Microstructure design plays a crucial role in regulating the microwave dielectric properties of materials, however, the understanding of frequency temperature stability and related micromechanism remains limited. In this study, a combination of first-principles calculations and experimental observation was used to investigate the correlation among sintering behavior, crystal structure, bonding nature, and microwave dielectric properties of LnPO(4) (Ln = Eu, Pr) ceramics. The research findings systematically clarify the optimized effect and micromechanism of lanthanides on the dielectric properties of monazite ceramics, providing insights into the design and enhancement of microwave dielectric materials.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Wenqian Pan, Xizhen Xia, Wei Zhou, Yang Li
Summary: The study investigates the frictional and wear behaviors of carbon fiber-reinforced SiC ceramic matrix composites with different fiber orientations mating with ceramic balls. The results show that fiber orientation significantly affects the friction and wear properties of the composites. Pads with randomly arranged fibers demonstrate better friction stability and lower wear volume, potentially suitable for bearing material applications. The research also explores the factors influencing the formation of continuous tribo-film and identifies abrasive wear and oxidation wear as the dominant wear mechanisms for the friction pairs.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Sergey Nikolaevich Perevislov, Ilya Evgenievich Arlashkin, Valentina Leonidovna Stolyarova
Summary: This paper describes the synthesis and sintering of MAX phases in the Zr-Al-C system. Different mixtures of initial Zr/Al/C and Zr/Al/ZrC powders were used to synthesize Zr2AlC and Zr3AlC2 MAX phases. The highest content of Zr3AlC2 MAX phase was obtained using a component ratio of 1:1.5:2-51.1 vol.% of Zr/Al/ZrC powders.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Weijia Luo, Xubin Wang, Baiheng Bai, Jianli Qiao, Xingcong Chen, Yongzheng Wen, Jingbo Sun, Lingxia Li, Ji Zhou
Summary: This study successfully establishes the relationship between internal strain and dielectric loss by synthesizing and designing specific structure of tungsten bronze ceramics, and concludes that controlling internal strain can effectively reduce dielectric loss. This research is of great significance for the development of future all-ceramic non-Hermitian devices.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Santanu Mondal, Juan Diego Shiraishi Lombard, Sreenivasulu Gollapudi, Carolina Tallon, Jie-Fang Li, Dwight Viehland
Summary: Ultrafast high-temperature sintering (UHS) is an effective method for rapidly densifying ZrB2 powders. The final grain size increases with longer sintering duration. X-ray diffraction and energy-dispersive spectroscopy show crystalline phase and compositional uniformity in ZrB2 after UHS.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
JiaNan Wang, ZhiQiang Li, YongZheng Zhu, Yao Liang, Yan Cui, HuaLong Tao, Bo Song, Alexander Nikiforov, ZhiHua Zhang
Summary: First-principles calculations were performed to investigate the crystal structure, electronic structure, and ion diffusion of sulfur-doped Li2FeSiO4. The results showed that sulfur doping can improve the electronic conductivity and reduce the energy barrier for ion diffusion.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Xiaodi Dai, Serdar Aydin, Mert Yuecel Yardimci, Gunter Reekmans, Peter Adriaensens, Geert De Schutter
Summary: This study investigates the rheological behavior, solidification process, and nanostructure changes of sodium hydroxide-activated slag (NH-AAS) and sodium silicate-activated slag (SS-AAS) pastes over time. The results show that NH-AAS and SS-AAS release similar heat and reach a similar reaction degree at their initial setting times, but have different gel structures.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Yanliang Ji, Simon Becker, Zichen Lu, Alexander Mezhov, Regine von Klitzing, Schmidt Wolfram, Dietmar Stephan
Summary: This study reveals the significant influence of resting time on the rheological properties of cement suspensions, which is closely related to non-absorbed polycarboxylate superplasticizers (PCEs) size variation. Adsorbed PCE during resting tends to bridge particles instead of dispersing them, leading to an increased yield stress.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Yifeng Huang, Xin Wang, Yinchang Ma, Xiang Lv, Jiagang Wu
Summary: This study investigates the effect of K/Na ratio on the phase structure, ferroelectric domains, and piezoelectric properties of potassium sodium niobate (KNN)-based ceramics. It reveals that high Na+ content leads to large ferroelectric domains, while high K+ content results in local polarity heterogeneity and distinct dielectric relaxational behavior. The balanced local polarity and stress heterogeneities contribute to improved piezoelectricity.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Zun Xia, Yedong Rong, Hao Li, Ye Dong, Hongbo Yu, Jie Xu, Xiuhui Wang, Jinlong Yang
Summary: This study presents the synthesis of hollow MgAl2O4 particles in situ within porous ceramics, resulting in volume expansion and the formation of a hierarchical pore structure, leading to a significant improvement in compressive strength.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)
Article
Materials Science, Ceramics
Honglong Wang, Zhiguo Sun, Faming Xia, Chenguang Yang, Xiaoguang Wang, Jintang Li, Linxu Jiang
Summary: In this study, the micro-geometry morphology variation and microstructural transformation mechanism of muscovite crystals under electron beam irradiation were explored. The results revealed the instability of the muscovite lattice under irradiation, as well as the expansion and shrinkage of the lattice with increasing dose. The study also identified changes in chemical structure and other mechanisms involved. These findings are significant for the design of radiation-resistant silicate materials and the manufacturing of electronic components used in the aerospace industry.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2024)