4.8 Article

Detection of an Unconventional Superconducting Phase in the Vicinity of the Strong First-Order Magnetic Transition in CrAs Using 75As-Nuclear Quadrupole Resonance

Journal

PHYSICAL REVIEW LETTERS
Volume 114, Issue 11, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.114.117002

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Funding

  1. Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan [22740231, 20102005, 24340085]
  2. Grants-in-Aid for Scientific Research [22740231, 26400359] Funding Source: KAKEN

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Pressure-induced superconductivity was recently discovered in the binary helimagnet CrAs. We report the results of measurements of nuclear quadrupole resonance for CrAs under pressure. In the vicinity of the critical pressure Pc between the helimagnetic (HM) and paramagnetic (PM) phases, a phase separation is observed. The large internal field remaining in the phase-separated HM state indicates that the HM phase disappears through a strong first-order transition. This indicates the absence of a quantum critical point in CrAs; however, the nuclear spin-lattice relaxation rate 1= T-1 reveals that substantial magnetic fluctuations are present in the PM state. The absence of a coherence effect in 1= T-1 in the superconducting state provides evidence that CrAs is the first Cr-based unconventional superconductor.

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