Journal
JOURNAL OF PHYSICAL CHEMISTRY B
Volume 112, Issue 2, Pages 558-567Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp075497e
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We derive the basic theoretical formulation for X-ray diffraction with pulsed fields, using a fully quantized description of light and matter. Relevant time scales are discussed for coherent as well as incoherent X-ray pulses, and we provide expressions to be used for calculation of the experimental diffraction signal for both types of X-ray sources. We present a simple analysis of time-resolved X-ray scattering for direct bond breaking in diatomic molecules. This essentially analytical approach highlights the relation between the signal and the time-dependent quantum distribution of internuclear positions, including thermal effects.
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