Journal
JOURNAL OF MATERIALS CHEMISTRY
Volume 21, Issue 17, Pages 6144-6147Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1jm10669d
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Funding
- Natural Science Foundation of China [21053001, 20701014, 50971063]
- Natural Science Foundation of Fujian Province of China [2010J01042]
- Fundamental Research Funds for the Central Universities [2009ZM0030]
- SRP program
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A new layer nitrogen-containing porous cerium trimetaphosphimate with pendant NH groups projecting into the channels has been synthesized and characterized. Knoevenagel condensation of benzaldehyde and ethyl cyanoacetate is carried out with this complex as support in ethanol at 333 K. Experimental results indicate that it is an efficient base catalyst. The NH groups are incorporated into the host framework and provide the base sites for catalysis. This stable solid base catalyst can be reused without obvious loss of its activity for three cycles.
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