Investigation of the non-linear loss properties of magnetic fluids subject to large alternating fields

The non-linear relaxational properties of a water-based magnetic fluid are investigated by means of measuring the frequency dependent complex susceptibility, chi(omega) in the presence of an external potential. The results obtained are discussed in terms of the magnetic analogue of the Coffey and Paranjape model as modified by Dejardin. The loss processes in the magnetic fluid in the non-linear region are investigated in the context of the loss tangent, tan(delta), and the power dissipation per unit volume. These measurements are of importance because of the continuing interest in the clinical applications of magnetic fluids, where large alternating magnetic fields can be applied to magnetic fluids to induce loss processes and heating effects, often driving the magnetic fluid into the non-linear region of magnetisation. We evaluate the increment of the susceptibility, Delta chi, due to the non-linear response, through measurement of chi(omega), and extend this formulism to the non-linear increment of the loss tangent, Delta tan(delta) and the increment of the heating rate, Delta U-heat. (C) 2007 Elsevier B. V. All rights reserved.