Article
Chemistry, Physical
Yao Xie, Guotao Sun, Jiwei Li, Renrui Sun, Lining Sun
Summary: This study investigates the luminescent properties of photoluminescent metal-organic frameworks (MOFs) doped with lanthanide ions. By selecting Er3+ and Y3+ ions as the metal centers and using Er3+ as a sensitizer, the MOFs are able to emit visible and near-infrared light. The variation of energy-transfer paths in the presence of different lanthanide activators is explored through the doping of Tm3+, Ho3+, and Eu3+ ions. This research provides new insights for the development of luminescence in MOFs.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2023)
Editorial Material
Energy & Fuels
Betar M. Gallant
Summary: By judiciously controlling the electrode interface and reactant transport, researchers have discovered a lower energy pathway for the direct conversion of captured CO2 to CO. This breakthrough may lead to more energy-efficient CO2 conversion processes.
Article
Physics, Multidisciplinary
Shun-Yao Zhang, Dong Yuan, Thomas Iadecola, Shenglong Xu, Dong-Ling Deng
Summary: This study proposes a matrix-product-state algorithm to extract nonthermal excited eigenstates in quantum many-body scarred systems, and applies it to various models, providing a new approach for future investigations of nonthermal excitations.
PHYSICAL REVIEW LETTERS
(2023)
Article
Chemistry, Physical
Anna Lucia Pellegrino, Emil Milan, Adolfo Speghini, Graziella Malandrino
Summary: In this study, Eu-doped CaF2 thin films were fabricated using the sol-gel process for down-shifting applications. The fine-tuning of parameters resulted in high uniformity films with good crystalline properties even at low temperatures. The down-shifting properties were validated through fluorescence measurements, and a correlation with doping ion percentages was observed.
Article
Physics, Multidisciplinary
Z. Chen, Y. Y. Tsui, M. Z. Mo, R. Fedosejevs, T. Ozaki, V. Recoules, P. A. Sterne, A. Ng
Summary: We report on the study of electron kinetics induced by intense femtosecond laser excitation of electrons in the 5d band of Au. Changes in electron system are observed from the temporal evolution of ac conductivity and conduction electron density. The results reveal an increase of electron thermalization time with excitation energy density, contrary to the Fermi-liquid behavior, and uncover the shortening of 5d hole lifetime with the increase of photoexcitation rates, providing valuable insights for understanding electron kinetics under extreme nonequilibrium conditions.
PHYSICAL REVIEW LETTERS
(2021)
Article
Multidisciplinary Sciences
Jie Ye, Chao Wang, Chao Gao, Tao Fu, Chaohui Yang, Guoping Ren, Jian Lu, Shungui Zhou, Yujie Xiong
Summary: This study presents a novel biotic-abiotic hybrid system that combines NiCu alloys with CdS semiconductors and Methanosarcina barkeri, achieving efficient methane production while reducing the side product of H-2. This work provides important insights into the biotic-abiotic interface and offers a new approach for engineering the process of methane generation.
NATURE COMMUNICATIONS
(2022)
Article
Chemistry, Physical
Zhengce An, Jinshu Huang, Long Yan, Li He, Bo Zhou
Summary: Persistent luminescence has become a hot research topic with various applications. However, most reported persistent luminescence is based on dopants rather than the host matrix, which also plays an important role. This study presents a novel nanostructure design that combines persistent luminescence, upconversion, and down-shifting luminescence to control emission colors under different excitation modes. Additionally, the physical origin of persistent luminescence in the CaF2 matrix is explored through simulations of energy band structures and defects.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2022)
Article
Materials Science, Multidisciplinary
Kensuke Tamura, Hosho Katsura
Summary: We introduce a class of spinless fermion models that exhibit quantum many-body scars originating from density-assisted hopping. We construct exact eigenstates with finite energy density and analyze their nonthermal nature through entanglement entropy and correlation functions. We investigate the dynamics from specific initial states and confirm the nonthermalizing dynamics induced by the quantum many-body scars. Furthermore, we provide a parent Hamiltonian with the quantum many-body scars as unique ground states and offer a rigorous proof for their uniqueness.
Article
Physics, Fluids & Plasmas
Dibyendu Roy, Divij Mishra, Tomaz Prosen
Summary: In this study, we investigate the spectral form factor in periodically kicked bosonic chains. By using the random phase approximation, we demonstrate that the spectral form factor can be rewritten in terms of a bistochastic many-body process generated by an effective bosonic Hamiltonian. This research provides important insights into the system size effects and the relationship between particle number and spectral properties.
Article
Physics, Fluids & Plasmas
Jae Sung Lee, Joonhyun Yeo
Summary: In this study, we investigate the Lindbladian quantum master equations (QMEs) and compare them with the Redfield equation. We find that the steady states of Lindbladian QMEs are different from the mean force Gibbs (MFG) state, especially when enforcing complete positivity. Furthermore, in the high-temperature regime, both the steady states of Lindbladian QMEs and the MFG state can be reduced to the Gibbs state of the system Hamiltonian under certain conditions.
Article
Physics, Fluids & Plasmas
Jason Iaconis, Andrew Lucas, Rahul Nandkishore
Summary: Subdiffusion is observed in chaotic many-body dynamics with multipole conservation laws and subsystem symmetries, as studied through numerical simulations of quantum automaton random unitary circuits. The results align well with recent hydrodynamic predictions for such theories.
Editorial Material
Chemistry, Physical
Ken Caldeira, Jacqueline A. Dowling
Summary: In a modeling study published in Energy & Environmental Science, researchers found that a portfolio of energy storage technologies is the most cost-effective way to ensure reliable electricity supply in the face of variability in wind and solar generation and electricity demand.
Article
Physics, Particles & Fields
Mohammad Ali-Akbari, Mahsa Lezgi
Summary: In this study, holographic subregion complexity is investigated in a spatially anisotropic field theory. A new interpretation from the informational perspective is proposed to determine the stable and unstable thermodynamically solutions. The effect of anisotropy on holographic subregion complexity is observed to be decreasing.
EUROPEAN PHYSICAL JOURNAL C
(2022)
Article
Physics, Multidisciplinary
Bjarne Bergh, Martin Gaerttner
Summary: Entanglement is a crucial resource for many quantum technologies and fundamental physics questions. This text discusses deriving measurable lower bounds on distillable entanglement using entropic uncertainty relations for bipartite systems, and showcases their application to physical models realizable in cold-atom experiments. The derived entanglement bounds rely on measurements in only two different bases and are generically applicable to any quantum simulation platform.
PHYSICAL REVIEW LETTERS
(2021)
Article
Thermodynamics
Sean A. Myers, Hongxi Li, Gabor A. Csathy
Summary: The article discusses the issue of ruthenium oxide resistance thermometers losing sensitivity at the lowest temperatures achieved in dilution refrigerators, and introduces a new thermometer design and the role of the key component, an in situ radio frequency filter. The study found that encasing the filter in an rf-tight enclosure is crucial for mitigating parasitic heating effects.