Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 13, Issue 21, Pages 5880-5884Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ob00619h
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Funding
- National Basic Research Program of China (973 Program) [2011CB808600]
- National Natural Science Foundation of China [21322203, 21272238, 21472194]
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A dehydrogenative olefination of C(sp(3))-H bonds is disclosed here, by merging rhenium catalysis with an alanine-derived hypervalent iodine(III) reagent. Thus, cyclic and acyclic ethers, toluene derivatives, cycloalkanes, and nitriles are all successfully alkenylated in a regio- and stereoselective manner.
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