Journal
JOURNAL OF COORDINATION CHEMISTRY
Volume 65, Issue 7, Pages 1144-1157Publisher
TAYLOR & FRANCIS LTD
DOI: 10.1080/00958972.2012.666349
Keywords
Manganese(III)tetraphenylporphyrin; Alkene epoxidation; Sodium periodate; Multi-wall carbon nanotubes; Heterogeneous catalyst
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Funding
- Center of Excellence of Chemistry of University of Isfahan (CECUI)
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Manganese(III)tetraphenylporphyrin supported on multi-wall carbon nanotubes (MWCNTs) were developed as efficient catalysts for epoxidation of alkenes with sodium periodate under mild conditions. The catalysts were prepared by axial ligation of manganese to 2-aminobenzimidazole and 2-aminothiazole preanchored to MWCNTs. The formation of these heterogenized catalysts was followed using elemental analysis, FT-IR spectroscopy, diffuse reflectance UV-Vis spectrophotometry, and scanning electron microscopy. The reactivity of these catalysts under both magnetic stirring and ultrasonic irradiation and also their reusability were investigated.
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