Article
Optics
Xinlin Lv, Junchi Chen, Yujie Peng, Yingbin Long, Guanting Liu, Yuxin Leng
Summary: In this study, a high-energy all-solid-state extracavity Raman oscillator and a high-energy single-pass Raman generator based on KGW crystal were investigated both theoretically and experimentally. The results showed the performance of these Raman laser structures under different pumping laser energies, demonstrating their potential applications in high-energy solid-state Raman lasers.
OPTICS AND LASER TECHNOLOGY
(2021)
Article
Optics
Yuxi Jia, Chencheng Shen, Xianglong Cai, Jinbo Liu, Tiancheng Zheng, Ming Xu, Dong Liu, Jingwei Guo
Summary: Nitrogen was used as an active gas to generate laser beams at 1415 nm and 2110 nm through Raman scattering. By optimizing parameters, the pulse energy and peak power of the lasers were successfully increased.
OPTICS COMMUNICATIONS
(2023)
Review
Chemistry, Analytical
Adriana Adamczyk, Sylwia Orzechowska, Anna Maria Nowakowska, Krzysztof Brzozowski, Katarzyna Majzner, Malgorzata Baranska
Summary: This article presents the recent advances in using stimulated Raman scattering (SRS) microscopy for spectroscopic analysis of cancer cells to identify pathological changes and understand the mechanism of metastasis. SRS microscopy, with its stronger signals and ability to time-resolve vibrational motions, offers rapid analysis of single cells. The article showcases the development of modern Raman imaging technology based on nonlinear optics and its application in analyzing various tumor cells, particularly leukemia.
TRAC-TRENDS IN ANALYTICAL CHEMISTRY
(2023)
Article
Chemistry, Analytical
Hongli Ni, Peng Lin, Yifan Zhu, Meng Zhang, Yuying Tan, Yuewei Zhan, Zian Wang, Ji-Xin Cheng
Summary: This study introduces a compact fiber laser-based multiwindow SRS imaging system that addresses issues with bulky and environmentally sensitive solid-state OPO, and slow wavelength tuning speed, demonstrating high-quality SRS metabolic imaging across various Raman windows.
ANALYTICAL CHEMISTRY
(2021)
Article
Optics
A. Yu Pyatyshev, A. Skrabatun, A. Vodchits
Summary: This study shows for the first time that rectified ethanol can be effectively used for converting laser radiation into different spectral ranges through stimulated Raman scattering (SRS), which is observed upon excitation by ultrashort pulses of a YAG:Nd3+ laser operated at a wavelength of 355 nm.
Article
Crystallography
Jian-Cheng Chen, Yu-Wen Ho, Yueh-Chi Tu, Hsing-Chih Liang, Yung-Fu Chen
Summary: A novel scheme was developed for a diode-pumped passively Q-switched Nd:YVO4/KGW Raman laser at 589 nm with a diode-to-orange conversion efficiency reaching 11.4%. The compact near-concentric cavity was designed to achieve good passive Q-switching and contain a coupled resonator for intracavity stimulated Raman scattering (SRS) and second harmonic generation (SHG). The dependence of the output performance on the initial transmission of the saturable absorber was explored, and the influence of the pump-to-mode size ratio was also considered.
Article
Materials Science, Multidisciplinary
Peng Lei, Xin Ding, Yuntao Bai, Xuanyi Yu, Guoxin Jiang, Tengteng Li, Bing Sun, Xingrui Zhang, Xiangxiang Li, Liang Wu, Guizhong Zhang, Jianquan Yao
Summary: The study demonstrated an efficient MgO:PPLN singly resonant optical parametric oscillator pumped by a Nd:YVO4/YVO4 laser, achieving high conversion efficiency and output power with excellent optical performance. The tuning range of the signal wave can be achieved by adjusting the crystal period.
RESULTS IN PHYSICS
(2021)
Article
Spectroscopy
Imaiyan Chitra Ragupathy, Volker Schweikhard, Andreas Zumbusch
Summary: Coherent Raman scattering microscopy is a new technology for label-free imaging, offering the possibility to record hyperspectral data. Multivariate methods outperform univariate analysis for the analysis of hyperspectral SRS data. Among the methods tested, multivariate curve resolution (MCR) gives the best results, showing a simple workflow for the analysis of hyperspectral coherent Raman imaging data.
JOURNAL OF RAMAN SPECTROSCOPY
(2021)
Article
Engineering, Electrical & Electronic
A. L. Koromyslov, I. M. Tupitsyn, E. A. Cheshev, R. Chulkov
Summary: In a solid-state inhomogeneously diode end-pumped Nd:KGW/Cr4+:YAG laser, lasing is achieved at wavelengths of 1067 and 1181 nm under conditions of frequency degeneracy. The characteristic ring spatial structure of radiation indicates transverse mode locking of the fundamental and Stokes components. By changing the position of an undoped KGW crystal in the cavity, the Raman conversion efficiency can be controlled, showing that transverse mode locking is accompanied by total longitudinal mode locking at lambda = 1067 and 1181 nm.
QUANTUM ELECTRONICS
(2021)
Article
Optics
Nicola Coluccelli, Giovanni Cichelli, Paolo Laporta, Giulio Cerullo
Summary: We propose a system that combines a high-energy femtosecond ytterbium laser, an optical parametric amplifier, and a photonic crystal hollow core fiber compressor for coherent anti-Stokes Raman scattering spectroscopy. The use of the compressor allows for matching the duration of the Stokes pulse to that of the pump pulse, resulting in improved excitation efficiency. Experimental results and a theoretical model are presented to quantify the expected sensitivity improvement. The system is successfully demonstrated for detecting bacterial spores on a surface with a single laser shot, achieving an unprecedented signal-to-noise ratio.
Article
Spectroscopy
Christian T. Graefe, David Punihaole, Michael J. Lynch, W. Ruchira Silva, Renee R. Frontiera
Summary: The research team successfully implemented super-resolution techniques based on Raman spectroscopy, achieving signal depletion and spatial resolution enhancement. By adapting the laser system for soft matter samples with increased repetition rate, they demonstrated improved imaging capabilities. However, despite lowering pulse powers, significant improvements in resolution were not achieved.
JOURNAL OF RAMAN SPECTROSCOPY
(2021)
Article
Instruments & Instrumentation
Nao Hirai, Yasuhiro Maeda, Kosuke Hashimoto, Bibin B. Andriana, Hiroko Matsuyoshi, Hidetoshi Sato
Summary: The study introduces a new type of CARS instrument with a double-wavelength-emission, background-free, electronically tuned Ti:sapphire laser (DW-ETL), which can provide stable CARS spectra for biological applications by controlling each laser pulse emission throughout the fingerprint region.
APPLIED SPECTROSCOPY
(2021)
Article
Nanoscience & Nanotechnology
Yuanchao Liu, Jie Pan, Guobin Zhang, Binbin Zhou, Zebiao Li, Pikting Cheung, Weiliang Wang, Yuying Zhu, Siyi Xiao, Lianbo Guo, Condon Lau
Summary: This article proposes a substrate-free strategy to suppress the coffee ring effect, enrich analytes, and self-assemble a signal-amplifying platform for multimode laser sensing. The platform can dramatically enrich analytes and enables ultrasensitive multimode laser sensing.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Optics
Ting Zhang, Xiaohong Hu, Ran Pan, Zhenguang Wang, Wei Zhang, Yashuai Guo, Ye Feng, Yishan Wang, Wei Zhao
Summary: We demonstrated a more than 30 W all-fiber supercontinuum source by pumping a four-mode graded-index multimode fiber (GIMF) with around 5 picoseconds laser pulse. The discrete spectral peaks in the range of 350-700 nm were found to be generated by the geometric parametric instability effect and quasi-phase matched harmonic generation, while the spectral broadening from 700 nm to 1750 nm (and even to 2400 nm) was caused by the radiation of dispersive waves, stimulated Raman scattering, and the effects of optical soliton. Furthermore, an experimental comparison between the four-mode GIMF and the 50/125 standard GIMF showed that the wavelengths radiated by the parametric instability differed due to different dispersion values, and the supercontinuum generated by the four-mode GIMF had a flatter spectral profile and a wider wavelength range.
OPTICS AND LASER TECHNOLOGY
(2023)
Article
Optics
Alexey G. Kuznetsov, Sergey I. Kablukov, Yuri A. Timirtdinov, Sergey A. Babin
Summary: This article presents recent experimental results on the pulsed regimes of Raman conversion in multimode graded-index fibers. Different linear cavities for Raman fiber laser with modulation of losses or gain are explored and compared. The experiments show that nanosecond pulses can be observed under mode-locking conditions, with greatly improved beam quality compared to the pump diode.