4.6 Article

Undamped ultrafast pulsation of plasmonic fields via coherent exciton-plasmon coupling

Journal

NANOTECHNOLOGY
Volume 26, Issue 8, Pages -

Publisher

IOP PUBLISHING LTD
DOI: 10.1088/0957-4484/26/8/085202

Keywords

quantum dots; metallic nanoparticles; plasmon pulses; quantum coherence; excitons; decoherence

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We show that under certain conditions the plasmonic field of a hybrid system consisting of a metallic nanoparticle and a semiconductor quantum dot can be converted into ultrashort stationary pulses with temporal widths as short as 300 ps. This happens as this system interacts with an infrared and visible laser fields, both with time-independent amplitudes. These fields generate quantum coherence via simultaneous interband and intersubband transitions of the quantum dot, forcing the polarization dephasing rate of the quantum dot to become negative during the plasmon pulses. This makes the amplitudes of such pulses time-independent (undamped), indicating total suppression of quantum decoherence of the quantum dot. These results suggest that hybrid quantum dot-metallic nanoparticle systems can act as undamped coherent-plasmonic oscillators.

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