Journal
MACROMOLECULAR RAPID COMMUNICATIONS
Volume 37, Issue 1, Pages 67-72Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/marc.201500548
Keywords
1,4-polyisoprene; cyclodextrin; free radical polymerization; polyrotaxanes; slide ring gels
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Funding
- Deutsche Forschungsgemeinschaft [WE 1090/17-1]
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Synthesis of a cyclodextrin (CD) polyrotaxane is achieved for the first time by simultaneous free radical polymerization of isoprene, threading by CD, and stoppering by copolymerization of styrene. This reaction is performed in an eco-friendly manner in an aqueous medium similar to classical emulsion polymerization. Threaded CD rings of the polyrotaxane are cross-linked by hexamethylene diisocyanate, leading to highly elastic slide-ring gels.
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