Journal
HETEROCYCLES
Volume 86, Issue 2, Pages 947-954Publisher
Japan Inst Heterocyclic Chemistry
DOI: 10.3987/COM-12-S(N)96
Keywords
gamma-Alkylidene-gamma-butyrolactone; Dendrimer; Intramolecular Cyclization; gamma-Acetylenic Acid
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Funding
- Japan Society for the Promotion of Science (JSPS) [23656514]
- Grants-in-Aid for Scientific Research [23360357, 23656514] Funding Source: KAKEN
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Polyamine dendrimer-encapsulated Pd2+ catalysts were prepared by complexation of PdCl2 with internal tertiary amino groups of the dendrimer. The fifth-generation Pd2+ dendrimer catalyst showed cooperative catalysis between Pd2+ species and the internal nanocavity consisting of regularly arranged tertiary amino groups to promote the intramolecular cyclization of gamma-acetylenic acids efficiently.
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