4.6 Article

Study of the electroplating mechanism and physicochemical proprieties of deposited Ni-W-Silicate composite alloy

期刊

ELECTROCHIMICA ACTA
卷 117, 期 -, 页码 443-452

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2013.11.159

关键词

Ni-W alloy; Silicate; EQCM; GDOES; Electrodeposition

资金

  1. Action Integree Franco-Tunisienne du Ministere des Affaires Etrangeres et Europeennes francais et du Ministere de l'Enseignement Superieur, de la Recherche Scientifique et de la Technologie tunisien

向作者/读者索取更多资源

In this work, layers based on Nickel-Tungsten (Ni-W) were electroplated from citrate-ammonia bath with and without silicate addition. Firstly, Electrochemical Quartz Crystal Microbalance (EQCM) and Global Discharge Optical Emission Spectroscopy (GDOES) were used to investigate the electroplating mechanism of both coatings. The gain mass was 14 and 4.13 mu g cmaZ(-2) for Ni-W-SiI and Ni-W coatings, respectively Secondly, the morphology of the composite alloy shows a smooth and homogenous surface with compact cauliflower like-structure identified as silicate incorporation. Finally, after a long immersion into chloride solution, Ni-W-SiI composite film showed a good surface stability and a remarkable mechanical hardness. These proprieties enhanced the electrochemical behavior of the composite alloy. (C) 2013 Elsevier Ltd. All rights reserved.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.6
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Environmental Sciences

Modelization and implementation of free adsorption and electrosorption of Cr (VI) from wastewater using Al2O3 nanoparticles: assessment and comparison of the two processes

Wafa Sassi, Hana Boubaker, Hayet Ben-Khaled, Sana Dhaoui, Achraf Ghorbal, Jean-Yves Hihn

Summary: The study aimed to enhance the adsorption capacity of nanoparticles, shorten the purification time and cost of contaminated waters using electrosorption technique. Results showed that adsorption of Cr (VI) on nano-Al2O3 occurred on a homogenous surface, and electrosorption process had a higher adsorption yield compared to free adsorption. However, the electrosorption process caused the loss of crystallinity in Al2O3 nanoparticles.

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2021)

Letter Dermatology

Generalized ulcerative cutaneous sarcoidosis: an unusual presentation of the disease

Meryam Chaabani, Wissem Hafsi, Fatima Alaoui, Wiem Sassi, Mourad Mokni

INTERNATIONAL JOURNAL OF DERMATOLOGY (2022)

Article Electrochemistry

Prediction and optimization of electroplated Ni-based coating composition and thickness using central composite design and artificial neural network

Wafa Sassi, Mouna Mrad, Debasis Behera, Salah Ammar, Jean-Yves Hihn

Summary: The study used an artificial neural network and central composite design model to determine the optimal electroplating conditions for Ni-based alloys, including current density, pH, and temperature. The theoretically optimal conditions were found to be 42 mA cm(-2) current density, pH 4.5, and 50 degrees Celsius. XPS and XRD analyses showed that these conditions would result in homogeneous and compact alloy structures, as well as stable Ni-alloy crystallinity.

JOURNAL OF APPLIED ELECTROCHEMISTRY (2021)

Letter Dermatology

Pustular rash triggered by Pfizer-BioNTech COVID-19 vaccination: A case report

Meriem Rouai, Malek Ben Slimane, Wiem Sassi, Fatima Alaoui, Ines Chelly, Mourad Mokni

DERMATOLOGIC THERAPY (2022)

Article Medicine, General & Internal

Palmoplantar keratoderma: An unusual manifestation of hypohydrotic ectodermic dysplasia

Wissal Abdelli, Asmahen Souissi, Fatima Alaoui, Wiem Sassi, Ines Chelly, Slim Haouat, Mourad Mokni

Summary: Rapp-Hodgkin syndrome (RHS) is a rare condition characterized by ectodermal dysplasia and palatal abnormalities. This case report describes a 15-year-old boy with RHS associated with palmoplantar keratoderma (PPK).

CLINICAL CASE REPORTS (2022)

Article Chemistry, Applied

Optimization and comparison study of adsorption and photosorption processes of mesoporous nano-TiO2 during discoloration of Indigo Carmine dye

Imen Ghanmi, Wafa Sassi, Paula Oulego, Sergio Collado, Achraf Ghorbal, Mario Diaz

Summary: This study focuses on the removal of Indigo Carmine dye using synthetic mesoporous Titanium dioxide nanoparticles, and determines the optimal contact time and adsorption capacity through process optimization. The study also analyzes the properties of reactors and thermodynamics.

MICROPOROUS AND MESOPOROUS MATERIALS (2022)

Article Chemistry, Multidisciplinary

Facile diazonium modification of pomegranate peel biochar: a stupendous derived relationship between thermal and Raman analyses

Ahmed M. Khalil, Radhia Msaadi, Wafa Sassi, Imen Ghanmi, Remy Pires, Laurent Michely, Youssef Snoussi, Alexandre Chevillot-Biraud, Stephanie Lau-Truong, Mohamed M. Chehimi

Summary: This study focuses on the modification of biochar derived from agricultural wastes through phosphoric acid treatment and arylation organic reaction. The results reveal that the arylation process has minimal impact on the morphology of the biochar, and the degree of arylation is highest at a specific concentration. Additionally, this study presents the first report on the diazonium modification of agrowaste-derived biochar and its potential applications.

CARBON LETTERS (2022)

Article Green & Sustainable Science & Technology

Pomegranate peel-derived biochar as ecofriendly adsorbent of aniline-based dyes removal from wastewater

Wafa Sassi, Imen Ghanmi, Paula Oulego, Sergio Collado, Salah Ammar, Mario Diaz

Summary: In this study, biochar derived from pomegranate peels was used for the first time as an adsorbent to remove aniline dyes. The optimum conditions for the adsorption of Aniline Yellow (AY) and Aniline Blue (AB) were determined using Artificial Neural Network and Central Composite Design modelization. The adsorption of AY and AB was found to be physical and spontaneous, with different thermodynamic properties. The application of the optimum conditions resulted in highly selective adsorption with percentages up to 95%.

CLEAN TECHNOLOGIES AND ENVIRONMENTAL POLICY (2023)

Article Polymer Science

Designing of anti-corrosive poly (γ-glycidoxypropyltriethoxysilane)-coated aluminum alloy via electro-polymerization: effect of cerium nitrate concentration

Mouna Mrad, Wafa Sassi, Jean-Yves Hihn, Fatima Montemor

Summary: This study evaluates the impact of cerium nitrate as an additive on the physico-chemical and anti-corrosion properties of sol-gel gamma-glycidoxypropyltriethoxysilane polymers (GPS) applied onto AA2024-T3 aluminum alloy. The addition of Ce(NO3)3 affects the morphology, chemical composition, and thickness of the electrodeposited coatings. Ce improves the anti-corrosion performance of GPS film, particularly at a concentration of 3.3 x 10(-2) M, by forming protective Ce oxides/hydroxides and blocking corrosion activity.

POLYMER BULLETIN (2023)

Article Environmental Sciences

Adsorption and Photocatalysis Properties of Perlite During Oxytetracycline Removal

Najeh Ardhaoui, Wafa Sassi, Radhia Msaadi, Nicolas Rouge, Salah Ammar, Ayman Nafady, Jean-Yves Hihn

Summary: This investigation explores the use of natural perlite mineral for removing oxytetracycline from aqueous solutions. The study analyzes the effects of contact time, initial concentration, and temperature on the removal efficiency. Kinetics of the adsorption process are studied using pseudo-first order and pseudo-second order models. Isotherm models, including Langmuir and Freundlich, are employed to understand the adsorption behavior. A thermodynamic analysis is conducted to reveal the nature of the adsorption process. The study also evaluates the photocatalytic efficiency of perlite.

WATER AIR AND SOIL POLLUTION (2023)

Article Engineering, Environmental

Selective/simultaneous batch adsorption of binary textile dyes using amorphous perlite powder: aspects of central composite design optimization and mechanisms

Wafa Sassi, Radhia Msaadi, Najeh Ardhaoui, Salah Ammar, Ayman Nafady

Summary: Selective/simultaneous adsorption of Congo Red (CR) and Methylene Blue (MB) has been effectively achieved using amorphous perlite. Optimum conditions of 38 min contact time, 96 mg/L dye concentration, and 312 degrees K temperature resulted in high adsorption yields of 82.22% for CR and 96.65% for MB. The adsorption process was found to occur through intradiffusional mass transport onto the porous material. Thermodynamic parameters indicated an endothermic/spontaneous physisorption process. SEM-EDS characterization revealed the surface adsorption process, while FTIR analysis showed disruption of compound order and decreased crystallinity of the adsorbent after adsorption. Application of these conditions to real industrial wastewater demonstrated simultaneous adsorption at neutral pH and 312 degrees K, with selective adsorption of CR at pH 4 and MB at pH 9.

JOURNAL OF ENVIRONMENTAL HEALTH SCIENCE AND ENGINEERING (2023)

Article Chemistry, Multidisciplinary

Adsorption of Methyl Orange onto Perlite: Optimization, Adsorption Kinetics, and Thermodynamic Studies

Radhia Msaadi, Asma Yahia, Wafa Sassi, Salah Ammar

Summary: In this study, the adsorption of methyl orange dye onto expanded Perlite was investigated. The optimal conditions for contact time, dye concentration and temperature were determined to be 115 min, 65 mg/L and 311 K, respectively. The highest adsorption yield and capacity were found to be 82.22% and 195.27 mg/g, respectively. Kinetic, isotherm and thermodynamic studies revealed the adsorption process characteristics. EDS, SEM and FTIR analysis confirmed the adsorption of MO onto Perlite.

CHEMISTRY AFRICA-A JOURNAL OF THE TUNISIAN CHEMICAL SOCIETY (2023)

Article Materials Science, Multidisciplinary

Valorization of pomegranate peel balls as bioadsorbents of methylene blue in aqueous media

Radhia Msaadi, Wafa Sassi, Jean-Yves Hihn, Salah Ammar, Mohamed M. Chehimi

Summary: Pomegranate peel balls were evaluated as bioadsorbents for the removal of methylene blue dye from aqueous solutions. The adsorption followed pseudo-second order kinetics and the maximum adsorption capacity varied with temperature, with physical adsorption being the primary mechanism. The waste generated by pomegranate peel could be considered for future water filtration and environmental protection in countries where pomegranates are available.

EMERGENT MATERIALS (2022)

Article Chemistry, Multidisciplinary

Evolution of Electrochemical Behavior, Electrical Conductivity, and Microhardness of Electrodeposited W Coatings Enhanced by Ni During Long Immersion in 3% NaCl Media

Radhia Msaadi, Wafa Sassi, Jean-Yves Hihn, Patrice Bercot, ElMustafa Rezrazi, Salah Ammar

Summary: This paper investigates the detailed physical and electrochemical properties of electroplated W enhanced by massive Ni coatings, revealing that all coatings corrode in 3% NaCl solution, leading to uniform corrosion of the enhanced W coating, with the main corrosion products being NiO, Ni(OH)(2) and WO3.

CHEMISTRY AFRICA-A JOURNAL OF THE TUNISIAN CHEMICAL SOCIETY (2021)

Article Business, Finance

THE IMPACT OF ADOPTION OF THE XBRL ON THE DEVELOPMENT OF STOCK MARKETS

Wafa Sassi, Hakim Ben Othman, Khaled Hussainey

Summary: The study shows that the adoption of XBRL has a negative impact on the development of stock markets, indicating the need for strict policies and mechanisms to ensure successful implementation and stakeholder understanding.

ASIA-PACIFIC MANAGEMENT ACCOUNTING JOURNAL (2021)

Article Electrochemistry

Recent advances in Bio-mass by electrochemically strategies generated hydrogen gas production: Environmentally sustainable technologies innovation

Abdul Qayoom Mugheri, Shaista Khan, Ali Asghar Sangah, Aijaz Ahmed Bhutto, Muhammad Younis Laghari, Nadeem Ahmed Mugheri, Asif Ali Jamali, Arsalan Ahmed Mugheri, Nagji Sodho, Abdul Waheed Mastoi, Aftab Kandhro

Summary: Green hydrogen has the potential to transition to a pollution-free energy infrastructure. This study proposes a solution to produce hydrogen during the photoelectrochemical process, offering greater stability and control over chemical reactions. Techno-economic assessments show the efficiency and economic feasibility of co-producing value-added chemicals to enhance green hydrogen production.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

ACGNet: An interpretable attention crystal graph neural network for accurate oxidation potential prediction

Danpeng Cheng, Wuxin Sha, Qigao Han, Shun Tang, Jun Zhong, Jinqiao Du, Jie Tian, Yuan-Cheng Cao

Summary: LiNixCoyMn1-x-yO2 (NCM) is a critical cathode material for lithium-ion batteries in electric vehicles. The aging of cathode/electrolyte interfaces leads to capacity degradation and long-term cycle instability. A novel neural network model called ACGNet is developed to predict electrochemical stability windows of crystals, allowing for high-throughput screening of coating materials. LiPO3 is identified as a promising coating material with high oxidation voltage and low cost, which significantly improves the cycle stability of NCM batteries. This study demonstrates the accuracy and potential of machine learning in battery materials.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Enhanced electrochemical performance of CuO/NiO/rGO for oxygen evolution reaction

P. Mohana, R. Yuvakkumar, G. Ravi, S. Arunmetha

Summary: This study successfully fabricates a non-noble CuO/NiO/rGO nanocomposite and investigates its electrocatalytic performance for oxygen evolution reaction in alkaline environment. The experimental results demonstrate that the electrocatalyst exhibits high activity and good stability, offering a new synthetic approach for sustainable energy production.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Carbon nanofibers implanted porous catalytic metal oxide design as efficient bifunctional electrode host material for lithium-sulfur battery

Qiong Qu, Jing Guo, Hongyu Wang, Kai Zhang, Jingde Li

Summary: In this study, a bifunctional electrode host design consisting of carbon nanofibers implanted ordered porous Co-decorated Al2O3 supported on carbon nanotube film (CNTF) was proposed to address the shuttling effect of lithium polysulfides (LiPSs) and dendrite formation of metal lithium anode in lithium-sulfur (Li-S) batteries. The electrode exhibited excellent conductivity, efficient confinement of LiPSs, and catalytic conversion performance, resulting in high initial capacity and good capacity retention during cycling. As an anode, the electrode showed excellent Li+ diffusion performance and uniform lithium growth behavior, achieving a dendrite-free lithium electrode. The flexible pack cell assembled from these electrodes delivered a specific capacity of 972 mAh g(-1) with good capacity retention.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Spray coating of carbon nanoparticles as an effective and scalable method to enhance the performance of stainless steel anode in microbial electrochemical systems

Hong Zhang, Jin-Peng Yu, Chen Chen, Cheng-Yong Shu, Guang-Yu Xu, Jie Ren, Kai Cui, Wen-Fang Cai, Yun-Hai Wang, Kun Guo

Summary: Spray coating of acetylene black nanoparticles onto stainless steel mesh can enhance its biofilm formation ability and current density, making it a promising electrode material for microbial electrochemical systems. The spray coating method is simple, cost-effective, and suitable for large-size stainless steel electrodes.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Electrochemical properties of Li-rich ternary cathode material Li1.20Mn0.44Ni0.32Co0.04O2 and its oxygen-deficient phase

Binpeng Hou, Jingjin Chen, Li-Hong Zhang, Xiaowen Shi, Zizhong Zhu

Summary: The electrochemical performance of Li1.20Mn0.44Ni0.32Co0.04O2 and its oxygen-deficient phase Li1.20Mn0.44Ni0.32Co0.04O1.83 was studied through first-principles calculations. The results show that the oxygen-deficient phase has a higher theoretical capacity but lower voltage platform and higher chemical activity compared to the pristine phase.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Post-mortem analysis of the Li-ion battery with charge/discharge deterioration in high- and low-temperature environments

Yating Du, Sayoko Shironita, Daisuke Asakura, Eiji Hosono, Yoshitsugu Sone, Yugo Miseki, Eiichi Kobayashi, Minoru Umeda

Summary: This study investigates the effect of high- and low-temperature environments on the charge-discharge performance of a Li-ion battery. The deterioration mechanisms of the battery at different temperatures are analyzed through various characterization techniques. The results indicate that the battery performance deteriorates more significantly at a low-temperature environment of 5 degrees C compared to higher temperatures. The understanding of the deterioration mechanisms can contribute to the development of safer battery usage methods.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

A Co3O4-x/Co nanocomposite with synergistically enhanced electrochemical activity for reduction of nitrite to ammonia

Si-Si Shi, Zhi-Xiang Yuan, Fei Zhang, Ping Chen

Summary: In this study, a new nano-electrocatalyst was prepared, which exhibited superior electrocatalytic activity for the reduction of NO2- to ammonia in a neutral electrolyte, potentially due to the synergistic enhancement between Co3O4-x and Co.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Facile fabrication of NaOH nanorods on pencil graphite electrode for simultaneous electrochemical detection of natural antioxidants by deep eutectic solvent

Berna Dalkiran, Havva Bekirog

Summary: This study reports the use of deep eutectic solvents (DES) based on ethylene glycol and urea as low-cost and green electrolytes for enhancing electrochemical detection of natural antioxidants. The study successfully developed a disposable and effective electrochemical sensing platform for simultaneous determination of ascorbic acid (AA) and gallic acid (GA) using NaOH nanorods on a pencil graphite electrode. The proposed electrode showed improved analytical performance, with higher peak currents and shifted oxidation potentials in DES compared to BR buffer medium.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

A three-dimensional fibrous tungsten-oxide/carbon composite derived from natural cellulose substance as an anodic material for lithium-ion batteries

Sijun Ren, Jianguo Huang

Summary: In this study, a novel bio-inspired nanofibrous WO3/carbon composite was synthesized using a facile hydrothermal method. The three-dimensional network structure of the composite alleviated the volume expansion of WO3 nanorods and enhanced the charge-transport kinetics. The optimized composite exhibited superior lithium storage properties.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Stabilizing the dissolution kinetics by interstitial Zn cations in CoMoO4 for oxygen evolution reaction at high potential

Zhilong Zheng, Yu Chen, Hongxia Yin, Hengbo Xiao, Xiangji Zhou, Zhiwen Li, Ximin Li, Jin Chen, Songliu Yuan, Junjie Guo, Haibin Yu, Zhen Zhang, Lihua Qian

Summary: This study found that interstitial Zn cations in CoMoO4 can modulate the dissolution kinetics of Mo cations and improve the OER performance. The interstitial Zn cations can prevent the dissolution of Co cations at high potential, enhancing the durability of the catalyst.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Molecular insights on optimizing nanoporous carbon-based supercapacitors with various electrolytes

Xiaobo Lin, Shern R. Tee, Debra J. Searles, Peter T. Cummings

Summary: Molecular dynamics simulations using the constant potential method were used to investigate the charging dynamics and charge storage of supercapacitors. The simulations revealed that the water-in-salt electrolyte exhibited the highest charge storage and significantly higher capacitance on the negative electrode. The varying contributions of different electrode regions to supercapacitor performance were also demonstrated.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Interaction between bilirubin oxidase and Au nanoparticles distributed over dimpled titanium foil towards oxygen reduction reaction

Wiktoria Lipinska, Vita Saska, Katarzyna Siuzdak, Jakub Karczewski, Karol Zaleski, Emerson Coy, Anne de Poulpiquet, Ievgen Mazurenko, Elisabeth Lojou

Summary: The spatial distribution of enzymes on electrodes is important for bioelectrocatalysis. In this study, controlled spatial distribution of gold nanoparticles on Ti nanodimples was achieved. The efficiency of enzymatic O2 reduction was found to be influenced by the size of the gold nanoparticles and their colocalization with TiO2. The highest stability of enzymatic current was observed with the largest gold nanoparticles.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Electrochemical supercapacitor and water splitting electrocatalysis applications of self-grown amorphous Ni(OH)2 nanosponge-balls

Tariq M. Al-Hejri, Zeenat A. Shaikh, Ahmed H. Al-Naggar, Siddheshwar D. Raut, Tabassum Siddiqui, Hamdan M. Danamah, Vijaykumar V. Jadhav, Abdullah M. Al-Enizi, Rajaram S. Mane

Summary: This study explores a promising self-growth approach for the synthesis of nickel hydroxide (Ni(OH)2) nanosponge-balls on the surface of a nickel-foam (NiF) electrode. The modified NiF electrode, named Ni(OH)2@NiF, shows distinctive nanosponge-ball morphology and demonstrates excellent energy storage capability and electrocatalytic performance in both hydrogen and oxygen evolution reactions.

ELECTROCHIMICA ACTA (2024)

Article Electrochemistry

Versatile mixed ionic-electronic conducting binders for high-power, high-energy batteries

Rafael Del Olmo, Gregorio Guzman-Gonzalez, Oihane Sanz, Maria Forsyth, Nerea Casado

Summary: The use of Lithium-Ion Batteries (LIBs) is becoming increasingly extensive, and it is important to optimize the devices to achieve their maximum practical specific capacity. In this study, mixed ionic-electronic conducting (MIEC) binders based on PEDOT:PSS and PEDOT: PDADMA-TFSI were developed for Li-ion cathodes, and their performance was compared with conventional formulations. The influence of electrode formulations, including the addition of conducting carbon and an Organic Ionic Plastic Cristal (OIPC), was also analyzed. The proposed binders showed improved performance compared to conventional formulations with different electrolyte types and active materials.

ELECTROCHIMICA ACTA (2024)