期刊
ELECTROCHIMICA ACTA
卷 143, 期 -, 页码 129-134出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2014.07.106
关键词
TiO2; Hollow sphere; Dye-sensitized solar cells; Light-scattering
资金
- National Natural Science Foundation of China [21171084, 21365010]
- National Basic Research Program of China [2011CBA00701]
- Nature Science Foundation of Hainan Province [213015, 214022]
- Project of Hainan Applied Technology Research and Development [ZDXM2014098]
- Undergraduate Training Programs for Innovation and Entrepreneurship [cxcyxj201414]
TiO2 hollow spheres with outer diameter of 1.0-2.5 mu m and shell thickness of 200 nm are successfully prepared via a facile hydrothermal method without use of any template agent. The as-prepared TiO2 hollow spheres are crystalline of the anatase phase, and possess a specific surface area of 48 m(2) g(-1). A high power conversion efficiency of 7.68% is achieved for dye-sensitized solar cell (DSSC) based on TiO2 hollow sphere photoanode, representing a 16% efficiency boost over that of 6.65% achieved with the P25 based DSSC. Based on the optical investigation and electrochemical impedance measurement, the improved performance can be attributed to the enhanced light-scattering and the reduced interface recombination. Crown Copyright (C) 2014 Published by Elsevier Ltd. All rights reserved.
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