期刊
CHEMISTRY-AN ASIAN JOURNAL
卷 7, 期 11, 页码 2656-2661出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201200539
关键词
absorption; dyes; pigments; fluorescence; fluorescent probes; nitrogen heterocycles
资金
- Foundation for Polish Science [TEAM/2009-4/3]
New, strongly fluorescent benzo[1,2-d:4,5-d']bisimidazoles have been prepared by the reaction of Bandrowski's base with various aldehydes. Their structures were carefully designed to achieve efficient excited-state intramolecular proton transfer and good two-photon-absorption (2PA) cross-sections. Functional dyes that possessed both high fluorescence quantum yields and large Stokes shifts were prepared. A p-expanded D-A-D derivative that possessed Ffl=50?% and s2=230 GM in the spectroscopic area of interest for biological imaging is an excellent candidate as a fluorescent probe. Thanks to the presence of two reactive amino groups, such compounds can be easily transformed into probes for bioconjugation. All of these benzo[1,2-d:4,5-d']bisimidazoles were also strongly fluorescent in the solid state.
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