期刊
MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING
卷 107, 期 -, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.mssp.2019.104838
关键词
Bi2O3; Metal-organic framework; Graphene oxide; Photocatalytic activity
类别
资金
- National Natural Science Foundation of China [51146008]
A novel Bi2O3/MOF/GO composite photocatalyst was prepared by a facile method, and characterized by XRD, SEM, EDS, FT-IR, BET, UV-Vis DRS and PL spectrum. The as-prepared Bi2O3/MOF/GO composites displayed the standout photocatalytic activity towards the degradation of Rhodamine B (RhB) under visible light irradiation. The introduction of MOF and graphene oxide into semiconductor Bi2O3 enhanced the photocatalytic activity dramatically, and the topgallant composite referred to BCG-2, which showed the highest photocatalytic activity. In the light of the active species trapping experiments, the OH and O2- radicals were the two main active radicals in the photocatalytic tests. The enhanced photocatalytic performance is chiefly ascribed to the formation of the tight joint interface in Bi2O3/MOF/GO composites, among which GO with the excellent conductivity and MOF with the certain adsorption effect during the photodegradation process. This synergistic effect is propitious to the transfer and separation of photo-generated carriers. At the same time, the Bi2O3/MOF/GO composite photocatalyst can maintain a stable photocatalytic activity and structure after three cycles. Finally, the possible mechanism of photocatalytic degradation of RhB was put forward.
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