期刊
MACROMOLECULAR RAPID COMMUNICATIONS
卷 35, 期 3, 页码 303-308出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/marc.201300829
关键词
fluorescence probe; logic gate; PDA vesicles; stimuli- responsive
资金
- National Natural Science Foundation of China [51173176, 51273186, 21074123, 91027024]
- Chinese Academy of Sciences [kjcx2-yw-m11]
- Fundamental Research Funds for the Central Universities [WK2060200008]
Here, a novel multi-stimuli-responsive fluorescence probe is developed by incorporating spiropyran group into the coumarin-substituted polydiacetylene (PDA) vesicles. The fluorescence of PDA can be turned on upon heating, and can be quenched upon exposure to UV light irradiation or pH stimuli owing to the fluorescene resonance energy transfer (FRET) between the red-phase PDA and the open merocyanine (MC) form of spiropyran. Moreover, we have designed and experimentally realized a set of logic gate operations for the first time based on the fluorescence modulation of the designed system upon thermal, photo, and pH stimuli. This novel type of resettable logic gates augur well for practical applications in information storage, optical recording, and sensing in complicated microenvironments.
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