期刊
GREEN CHEMISTRY
卷 14, 期 12, 页码 3269-3272出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2gc36276g
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资金
- CSIR-UGC
A novel imidazolium ylide activated [4 + 1] annulation approach is described for the diastereoselective synthesis of bicyclic and tricyclic fused dihydrofurans in water. This cascade annulation presumably proceeds via a Michael reaction triggered zwitterion enolate followed by concomitant intramolecular cyclization. The methodology has distinction of being the first report on imidazolium ylide mediated [4 + 1] annulation in water as a unified greener approach involving an in situ base regeneration system and an alternative to pyridine ylide.
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