期刊
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
卷 2012, 期 11, 页码 2266-2272出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201101732
关键词
Nitrogen heterocycles; Cross-coupling; Amination; Copper
资金
- Presidium of the Russian Academy of Sciences [OKhNM-04]
Access to unsymmetrical secondary dihetarylamines through the Cu(OAc)(2)/2-acetylcyclohexanone catalyzed cross-coupling of s-tetrazinylamines with iodofurazans has been developed. The reaction displays good functional group tolerance, involving nitro, azido, and azo groups, which are critical for the construction of energetic materials. Both 3,6-disubstituted and annelated s-tetrazines react readily with iodofurazans to furnish the desired products.
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