期刊
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
卷 2011, 期 14, 页码 2692-2696出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201100112
关键词
Copper; Cross-coupling; Ligand design; N,O ligands; Heterocycles
资金
- 973 Program [2010CB933501, 2011CBA00502]
- National Natural Science Foundation of China [20971122]
- Chinese Academy of Sciences
A series of ten acylhydrazine- and acylhydrazone-type ligands were designed and synthesized. Their electronic and steric properties were easily modified and tuned by varying the substituents in the vicinity of the acylhydrazine and acylhydrazone units. The effect of ligands on the catalytic activity of Ullmann reactions was assessed by using a combination of these ligands with CuI. The catalytic system is very efficient for the C-N coupling reaction of azoles with aryl and heteroaryl bromides.
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