4.4 Article

Low-temperature dipolar echoes in amorphous dielectrics: Significance of relaxation and decoherence free two-level systems

期刊

EPL
卷 104, 期 5, 页码 -

出版社

IOP PUBLISHING LTD
DOI: 10.1209/0295-5075/104/57006

关键词

-

资金

  1. LINK Program of NSF
  2. Louisiana Board of Regents [NSF(2012)-LINK-65]
  3. Army Research Office [vv911NF-13-1-0186]
  4. European Community Research Infrastructures [228464]

向作者/读者索取更多资源

The theoretical model for dielectric echoes in amorphous solids at low temperatures has been developed and applied to the recent two- and three-pulse echo experimental data in borosilicate glass BK7 where the amplitude of dipolar echoes has been observed for unprecedentedly long delay times extending the experimental window for studying the decay by several orders of magnitude. We show that at long delay times the echo amplitude is determined by a small subset of two-level systems (TLSs) with negligible relaxation and decoherence because of their weak coupling to phonons. The universal statistics of coupling is obtained by assuming that different TLS elastic tensor components are almost independent. Under this assumption the echo decay can be described approximately by the power law time dependences with different powers at times shorter and longer than the typical TLS relaxation time. These predictions are in a very good agreement with the experimental data and can be used to extract TLS relaxation and decoherence rates from the echo experiments. Copyright (C) EPLA, 2013

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.4
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Chemistry, Physical

Ballistic Transport of Vibrational Energy through an Amide Group Bridging Alkyl Chains

Layla N. Qasim, E. Berk Atuk, Andrii O. Maksymov, Janarthanan Jayawickramarajah, Alexander L. Burin, Igor V. Rubtsov

JOURNAL OF PHYSICAL CHEMISTRY C (2019)

Article Chemistry, Multidisciplinary

2D/3D Heterostructure for Semitransparent Perovskite Solar Cells with Engineered Bandgap Enables Efficiencies Exceeding 25% in Four-Terminal Tandems with Silicon and CIGS

Saba Gharibzadeh, Ihteaz M. Hossain, Paul Fassl, Bahram Abdollahi Nejand, Tobias Abzieher, Moritz Schultes, Erik Ahlswede, Philip Jackson, Michael Powalla, Soren Schaefer, Michael Rienaecker, Tobias Wietler, Robby Peibst, Uli Lemmer, Bryce S. Richards, Ulrich W. Paetzold

ADVANCED FUNCTIONAL MATERIALS (2020)

Article Instruments & Instrumentation

Development of a novel calorimetry setup based on metallic paramagnetic temperature sensors

Andreas Reifenberger, Andreas Reiser, Sebastian Kempf, Andreas Fleischmann, Christian Enss

REVIEW OF SCIENTIFIC INSTRUMENTS (2020)

Article Chemistry, Physical

Crucial effect of transverse vibrations on the transport through polymer chains

Alexei Boulatov, Alexander L. Burin

JOURNAL OF CHEMICAL PHYSICS (2020)

Article Nanoscience & Nanotechnology

Thermal Stability and Cation Composition of Hybrid Organic-Inorganic Perovskites

Jonas A. Schwenzer, Tim Hellmann, Bahram Abdollahi Nejand, Hang Hu, Tobias Abzieher, Fabian Schackmar, Ihteaz M. Hossain, Paul Fassl, Thomas Mayer, Wolfram Jaegermann, Uli Lemmer, Ulrich W. Paetzold

Summary: Through investigating the impact of different cation compositions on the thermal stability of perovskite thin films, it was found that methylammonium-based perovskite thin films exhibited more pronounced decomposition, while the stoichiometry in methylammonium-free formamidinium lead iodide (FAPbI(3)) and formamidinium cesium lead iodide (FACsPbI(3)) thin films was more stable, demonstrating remarkable stability with no decline in power conversion efficiency under thermal stress at 85 degrees C for 1000 h.

ACS APPLIED MATERIALS & INTERFACES (2021)

Article Chemistry, Physical

Efficient Light Harvesting in Thick Perovskite Solar Cells Processed on Industry-Applicable Random Pyramidal Textures

Ahmed Farag, Raphael Schmager, Paul Fassl, Philipp Noack, Bianca Wattenberg, Torsten Dippell, Ulrich W. Paetzold

Summary: Light management is crucial for high-performance solar cells, including monolithic perovskite/Si tandem solar cells. This study presents high-efficiency perovskite solar cells processed on industry-applicable random pyramidal textures. These textured solar cells demonstrate improved light management compared to planar cells, with reduced reflectance and enhanced light trapping. Furthermore, the textured cells maintain high fill factor and open-circuit voltage, and exhibit improved current generation for all angles of incidence, making them advantageous for realistic irradiation conditions and bifacial applications.

ACS APPLIED ENERGY MATERIALS (2022)

Article Chemistry, Physical

Monolithic Two-Terminal Perovskite/CIS Tandem Solar Cells with Efficiency Approaching 25%

Marco A. Ruiz-Preciado, Fabrizio Gota, Paul Fassl, Ihteaz M. Hossain, Roja Singh, Felix Laufer, Fabian Schackmar, Thomas Feeney, Ahmed Farag, Isabel Allegro, Hang Hu, Saba Gharibzadeh, Bahram Abdollahi Nejand, Veronique S. Gevaerts, Marcel Simor, Pieter J. Bolt, Ulrich W. Paetzold

Summary: This study successfully fabricated high-efficiency perovskite/CIS tandem solar cells, showcasing the potential of monolithic two-terminal structure. By optimizing the techniques, a power conversion efficiency approaching 25% was achieved, setting the foundation for future improvements in efficiency.

ACS ENERGY LETTERS (2022)

Article Physics, Multidisciplinary

Integration of maXs-type microcalorimeter detectors for high-resolution x-ray spectroscopy into the experimental environment at the CRYRING@ESR electron cooler

Ph Pfaefflein, S. Allgeier, S. Bernitt, A. Fleischmann, M. Friedrich, Ch Hahn, D. Hengstler, M. O. Herdrich, A. Kalinin, F. M. Kroeger, P. Kuntz, M. Lestinsky, B. Loeher, E. B. Menz, T. Over, U. Spillmann, G. Weber, B. Zhu, Ch Enss, Th Stoehlker

Summary: This study reports the integration of novel magnetic microcalorimeter detectors developed within SPARC into the experimental environment of storage rings at GSI, Darmstadt. The modifications made to the detector allow for precision x-ray spectroscopy of stored heavy ions.

PHYSICA SCRIPTA (2022)

Article Energy & Fuels

Four-Terminal Perovskite/Copper Indium Gallium Selenide Tandem Solar Cells: Unveiling the Path to >27% in Power Conversion Efficiency

Thomas Feeney, Ihteaz M. Hossain, Saba Gharibzadeh, Fabrizio Gota, Roja Singh, Paul Fassl, Adrian Mertens, Ahmed Farag, Jan-Philipp Becker, Stefan Paetel, Erik Ahlswede, Ulrich W. Paetzold

Summary: This article presents a method to improve the efficiency of 4T perovskite/CIGS tandem solar cells, achieving a PCE of 27.3% through systematic optimization of the top semi-transparent PSC. Improvements in light management through the optimization of anti-reflection coatings and the development of transparent conductive oxides that incur very low parasitic absorption are crucial for maximizing efficiency.

SOLAR RRL (2022)

Article Materials Science, Multidisciplinary

Optimization of SnO2 electron transport layer for efficient planar perovskite solar cells with very low hysteresis

Abed Alrhman Eliwi, Mahdi Malekshahi Byranvand, Paul Fassl, Motiur Rahman Khan, Ihteaz Muhaimeen Hossain, Markus Frericks, Simon Ternes, Tobias Abzieher, Jonas A. Schwenzer, Thomas Mayer, Jan P. Hofmann, Bryce S. Richards, Uli Lemmer, Michael Saliba, Ulrich W. Paetzold

Summary: The use of a bilayer c(Li)-NP-SnO2 ETL can enhance electron extraction and charge transport properties for perovskite solar cells, reducing J-V hysteresis and improving stability PCE compared to single-layer or undoped bilayer ETLs.

MATERIALS ADVANCES (2022)

Article Chemistry, Multidisciplinary

Two birds with one stone: dual grain-boundary and interface passivation enables >22% efficient inverted methylammonium-free perovskite solar cells

Saba Gharibzadeh, Paul Fassl, Ihteaz M. Hossain, Pascal Rohrbeck, Markus Frericks, Moritz Schmidt, The Duong, Motiur Rahman Khan, Tobias Abzieher, Bahram Abdollahi Nejand, Fabian Schackmar, Osbel Almora, Thomas Feeney, Roja Singh, Dirk Fuchs, Uli Lemmer, Jan P. Hofmann, Stefan A. L. Weber, Ulrich W. Paetzold

Summary: This study successfully enhanced the efficiency and stability of inverted p-i-n structured perovskite solar cells using a dual passivation strategy, achieving high power conversion efficiency and good stability.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

Article Materials Science, Multidisciplinary

Revealing the internal luminescence quantum efficiency of perovskite films via accurate quantification of photon recycling

Paul Fassl, Vincent Lami, Felix J. Berger, Lukas M. Falk, Jana Zaumseil, Bryce S. Richards, Ian A. Howard, Yana Vaynzof, Ulrich W. Paetzold

Summary: The study establishes an analysis procedure to accurately determine the photon escape probability of perovskite films based on PL spectra, revealing higher (p) over bar (e) values than previously assumed. Applying the model to CH3NH3PbI3 films corrects previous estimates for internal luminescence quantum efficiency, showing more potential for reducing non-radiative recombination than initially thought.

MATTER (2021)

Article Materials Science, Multidisciplinary

Polaronic effect of a metal layer on variable range hopping

Ofek Asban, Alexander Burin, Alexander Shnirman, Moshe Schechter

Summary: This study investigates the impact of a metal plate on the variable range hopping conductivity of a two-dimensional electron-glass system. It reveals both static and dynamic effects, with the former increasing conductivity at very low temperatures and the latter suppressing phonon-assisted hopping and conductivity over a wider temperature range than the static effect. The findings provide insights into the behavior of electron-glass systems with external influences.

PHYSICAL REVIEW B (2021)

Article Chemistry, Physical

Triple-cation low-bandgap perovskite thin-films for high-efficiency four-terminal all-perovskite tandem solar cells

Somayeh Moghadamzadeh, Ihteaz M. Hossain, The Duong, Saba Gharibzadeh, Tobias Abzieher, Huyen Pham, Hang Hu, Paul Fassl, Uli Lemmer, Bahram Abdollahi Nejand, Ulrich W. Paetzold

JOURNAL OF MATERIALS CHEMISTRY A (2020)

Article Materials Science, Multidisciplinary

Many-body localization in spin chains with long-range transverse interactions: Scaling of critical disorder with system size

Andrii O. Maksymov, Alexander L. Burin

PHYSICAL REVIEW B (2020)

暂无数据