期刊
ENERGY & FUELS
卷 26, 期 4, 页码 2528-2538出版社
AMER CHEMICAL SOC
DOI: 10.1021/ef300079w
关键词
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资金
- Advanced Research Projects Agency-Energy (ARPA-E), U.S. Department of Energy [DE-AR0000084]
- DOE-NETL [DE-NT0005310]
A novel method for the postcombustion capture of CO2 from coal-fired power plants has been described utilizing an aminosilicone absorbent. 1,3-Bis(3-aminopropy1)-1,1,3,3-tetramethyldsiloxane (GAP-0) rapidly transforms from a low viscosity liquid to a friable solid upon exposure to CO2 in simulated flue gas. This material has excellent thermal stability, low vapor pressure, high CO2 loading capability, and a large dynamic CO2 capacity between rich and lean solvent loadings. Preliminary plant and process models assembled from experimental data show a decrease in parasitic energy loss from 30% to 18% when compared to the benchmark monoethanolamine (MEA) process and a concomitant lowering of the cost of electricity (COE) from 74% to 44% increase versus a plant without carbon capture.
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