期刊
ELECTROCHEMISTRY
卷 76, 期 2, 页码 140-143出版社
ELECTROCHEMICAL SOC JAPAN
DOI: 10.5796/electrochemistry.76.140
关键词
dye Sensitization; chlorophyll; photoelectrochemistry; solar cell; photosynthesis; energy conversion
Chlorin e6, a metal-free hydrophilic derivative of chlorophyll, was used as a sensitizer of mesoporous TiO2 film to construct a high-efficiency solar cell as a model for artificial photosynthesis. The cell exhibited wide spectral responsivity in the visible light region that resembles action spectrum of photosynthesis. Optimization of dye adsorption method by using co-adsorbing surfactant agents that suppress intermolecular aggregation of the dye achieved high energy conversion efficiency up to 4.3% under simulated sunlight of 100 mW cm(-2) intensity.
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