4.4 Article

Particulate organic carbon export fluxes and validation of steady state model of 234Th export in the Chukchi Sea

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.dsr2.2012.03.003

关键词

POC export flux; Organic carbon burial rate; Th-234/U-238 disequilibrium; Non-steady-state model

资金

  1. Tsinghua University Initiative Scientific Research Program [2010THZ07]
  2. Scientific Research Foundation of Third Institute of Oceanography, SOA [2011025, 2010011, 2010001]
  3. Youth Fund of SOA [2011531, 2012107]
  4. National Natural Science Foundation of China [40976116]
  5. Open Fund of the Key laboratory of Global Change and Marine-Atmospheric Chemistry, SOA [GCMAC0902]

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To evaluate the efficiency of biological pump and carbon sequestration content on Arctic shelf, estimations of POC export fluxes derived from Th-234/U-238 disequilibrium were made during the 3rd Chinese National Arctic Research Expedition (CHINARE-3) from July 12 to September 22, 2008. The Th-234 analysis was based on small volume MnO2 co-precipitation and beta-counting method. Great deficits of Th-234 to U-238 were observed widely over Chukchi shelf, with an average Th-234/U-238 activity ratio of 0.64 +/- 0.28, resulting from intense particle scavenging. The average POC export: fluxes in the entire study area, shelf and slope area were 24.9 +/- 23.3, 29.5 +/- 23.0 and 2.1 +/- 0.5 mmol C m(-2) d(-1), respectively, resulting in that 21% of the primary production on average was exported to the benthos. Comparing with steady state model, non-steady-state model was recommended to derive a more accurate particulate Th-234 export flux in a rapidly changing environment in the high latitude areas. (C) 2012 Elsevier Ltd. All rights reserved.

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