期刊
DALTON TRANSACTIONS
卷 42, 期 5, 页码 1333-1337出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2dt31698f
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资金
- Engineering and Physical Sciences Research Council [EP/H004823/1] Funding Source: researchfish
- EPSRC [EP/H004823/1] Funding Source: UKRI
The reactions of f-block silylamido N-heterocyclic carbene (NHC) complexes ([M(L)(N{SiMe3}(2))(2)], M = Y, Ce, and U, L = bidentate alkoxy-tethered NHC ligand) with CO and CO2 have been studied and compared to each other, to those of selected [M(L)(2)(N{SiMe3}(2))] complexes, and to those of [M(N{SiMe3}(2))(3)] to identify the effect of the labile NHC group on the small molecule activation chemistry. The small molecules COS and N2CPh2 have also been studied.
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