期刊
DALTON TRANSACTIONS
卷 -, 期 44, 页码 9794-9799出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b916488j
关键词
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资金
- National Natural Science Foundation of China [20732007, 20672122, 20973189, 50973125]
- Ministry of Science and Technology of China [2006CB806105, G2007CB808004, 2007CB936001, 2009CB220008]
- Bureau for Basic Research of the Chinese Academy of Sciences
Square-planar polypyridine platinum(II) complexes have been introduced into a silica/polymer matrix by covalent ligand modi. cation. The photophysical properties of the supported matrices are well retained as their model complexes, and the quantum yields for singlet oxygen (O-1(2)) generation are comparable with that of TPP (tetraphenylporphyrin) under similar conditions. A preliminary application in photosensitized oxidation indicates the silica/polymer-supported matrices are promising, which can be reused without loss of reactivity by a simple filtration. Moreover, the polymer-supported matrix exhibits excellent compatibility in various solvents.
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