期刊
CRYSTAL GROWTH & DESIGN
卷 8, 期 11, 页码 3917-3920出版社
AMER CHEMICAL SOC
DOI: 10.1021/cg800639x
关键词
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资金
- FEDER
- POCI (Portugal) [POCI-PPCDT/QUI/58377/2004]
- Fundacao para a Ciencia e a Tecnologia (FCT, Portugal)
- [SFRH/BPD/9309/2002]
A synthetic approach combining hydrothermal and ionothermal (eutectic mixture of choline chloride and malonic acid) procedures is proposed that allowed the isolation of the first lanthanide-organic frameworks with residues of 1,4-phenylenebis(methylene)diphosphonic acid (H(4)pmd), [Ln(Hpmd)(H2O)] (where Ln(3+) = Ce3+ and Pr3+), exhibiting an unprecedented trinodal topology with 3- and 8-connected nodes. The structural details were unveiled front singale-crystal X-ray diffraction and the materials were characterized using standard techniques.
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