期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 54, 期 33, 页码 9577-9580出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201504603
关键词
carbocycles; enynes; heterocycles; peroxides; radicals
资金
- Natural Science Foundation of China [21472039, 21172060]
- Hunan Provincial Natural Science Foundation of China [13JJ2018]
A new metal-free oxidative radical [2+2+1] carbocyclization of benzene-linked 1,n-enynes with two C(sp(3))H bonds adjacent to the same heteroatom is described. This method achieves two C(sp(3))H oxidative functionalizations and an annulation, thus providing efficient and general access to a variety of fused five-membered carbocyclic hydrocarbons.
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