期刊
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY
卷 23, 期 -, 页码 21-26出版社
ELSEVIER SCIENCE INC
DOI: 10.1016/j.jiec.2014.08.033
关键词
Coal tar; Naphthalene; MoP; Hydrogenation; Zeolite
资金
- National Programme on Key Basic Research Project [2012CB214905]
- National Science Fund for Excellent Young Scholars [21422607]
- National Natural Science Foundation of China [51104140]
MoP catalyst supported on HZSM-5, HBeta and HY were prepared by wet impregnation and temperature programmed reduction (H-2-TPR), applied for the conversion of naphthalene to tetralin, and characterized by XRD, SEM, TEM, BET, H-2-TPR, and NH3-TPD. Catalytic tests revealed the highest selectivity to tetralin was observed over MoP/HY with a naphthalene conversion of 85% and a tetralin selectivity of 99%. The effect of temperature and liquid hourly space velocity (LHSV) was also studied. Well dispersed and small particles of MoP, reduced pore size and weak acidity of HY contribute to enhanced catalytic activity and selectivity in conversion of naphthalene to tetralin. (C) 2014 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
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