期刊
CHEMICAL SOCIETY REVIEWS
卷 38, 期 9, 页码 2556-2564出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b807498b
关键词
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资金
- Middle Atlantic Regional Center of Excellence for Biodefense and Emerging Infectious Diseases Research [NIH NIAID-U54 AI057168]
- NIH National Institute of Neurological Disorders and Stroke [R21 NS055187-01]
- NIH K25 Career Development Award [K25EB007565]
Chemiluminescent-based detection is entrenched throughout the biosciences today, such as in blotting, analyte and protein quanti. cation and detection. While the biological applications of chemiluminescence are forever growing, the underlying principles of using a probe, an oxidizer and a catalyst (biological, organic or inorganic) have remained mostly unchanged for decades. Subsequently, chemiluminescence-based detection is fundamentally limited by the classical photochemical properties of reaction yield, quantum yield, etc. However, over the last 5 years, a new technology has emerged which looks set to fundamentally change the way we both think about and use chemiluminescence today. Metal surface plasmons can amplify chemiluminescence signatures, while low-power microwaves can complete reactions within seconds. In addition, thin metal films can convert spatially isotopic chemiluminescence into directional emission. In this forward looking tutorial review, we survey what could well be the next-generation chemiluminescent-based technologies.
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